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颗粒学报（英文版）
颗粒学报（英文版）

郭慕孙

双月刊

1674-2001

jcsp@home.ipe.ac.cn

010-82629146

100080

北京中关村北二条1号中科院过程所内

颗粒学报（英文版）/Journal China ParticuologyCSCDCSTPCD北大核心EISCI
查看更多>>本刊以创精品与国际化为办刊方针，旨在反映中国颗粒学研究的最新成果、及时追踪国际颗粒学领域的最新动态。学报主要刊登国内外颗粒学领域中的研究、工程和应用方面的优秀原始论文，包括颗粒测试与表征、颗粒制备与处理、流态化、气溶胶和超微颗粒等。本刊不仅设有论坛、研究论文、研究简报等内容，还有书评、会议信息与报道、测试仪器进展等栏目，便于相关人士进行学术交流，并为科技成果的展示提供平台，信息十分丰富。本刊已陆续被美国化学文摘（CA），俄罗斯文摘杂志（AJ），剑桥科学文摘（CSA）以及中国科技论文与引文数据库(CSTPCD)收录。China PARTICUOLOGY, a bimonthly interdisciplinary journal in English, purports to present the best papers in research, engineering and application in the overall field of PARTICUOLOGY, including particle characterization, particle preparation, aerosol, fluidization and ultra-fine particles. The word PARTICUOLOGY was coined to correspond to its Chinese terminology, which denotes both the science and technology of particles. Although the journal is China-based, it serves as a medium for all accepted papers of international origin, especially the best papers representing current advances in the world. Besides scientific and engineering papers, the journal includes the following sections: R & D notes, Current events, Editorials reviews, Forum for comments, opinions and qualified speculations, News on books, instruments and meetings.Now， China Particuology has been indexed by CA, AJ , CSA and CSTPCD.??读者对象（Audiences）： 中国颗粒学会会员、国内外从事颗粒学和颗粒技术研究和生产的大专院校师生、科研院所及企业的研究人员和技术人员。 Member of Chinese Society of Particuology, and researchers or experts who are engaged in the study of particle sciences and technology coming from colleges, institutes and corporations all over the world.
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    Experimental and numerical investigation to elucidate the fluid flow through packed beds with structured particle packings

    Shirin PatilChristian GorgesJoel Lòpez BonillaMoritz Stelter...
    218-237页
    查看更多>>摘要：The present paper presents an experimental and numerical investigation of the dispersion of the gaseous jet flow and co-flow for the simple unit cell(SUC)and body-centred cubic(BCC)configuration of particles in packed beds.The experimental setup is built in such a way that suitable and simplified boundary conditions are imposed for the corresponding numerical framework,so the simulations can be done under very similar conditions as the experiments.Accordingly,a porous plate is used for the co-flow to achieve the uniform velocity and the fully developed flow is ensured for the jet flow.The SUC and BCC particle beds consist of 3D-printed spheres,and the non-isotropy near the walls is mostly eliminated by placing half-spheres at the channel walls.The flow velocities are analysed directly at the exit of the particle bed for both beds over 36 pores for the SUC configuration and 60 pores for the BCC configuration,for particle Reynolds numbers of 200,300,and 400.Stereo particle image velocimetry is experimentally arranged in such a way that the velocities over the entire region at the exit of the packed bed are ob-tained instantaneously.The numerical method consists of a state-of-the-art immersed boundary method with adaptive mesh refinement.The paper presents the pore jet structure and velocity field exiting from each pore for the SUC and BCC packed particle beds.The numerical and experimental studies show a good agreement for the SUC configuration for all flow velocities.For the BCC configuration,some dif-ferences can be observed in the pore jet flow structure between the simulations and the experiments,but the general flow velocity distribution shows a good overall agreement.The axial velocity is generally higher for the pores located near the centre of the packed bed than for the pores near the wall.In addition,the axial velocities are observed to increase near the peripheral pores of the packed bed.This behaviour is predominant for the BCC configuration as compared to the SUC configuration.The velocities near the peripheral pores can become even higher than those at the central pores for the BCC config-uration.It is shown that both the experiments as well as the simulations can be used to study the complex fluid structures inside a packed bed reactor.
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    Lithium polysulfide solvation and speciation in the aprotic lithium-sulfur batteries

    Jinhao ZhangQingshan FuPeng LiRuibo Linghu...
    238-245页
    查看更多>>摘要：Fingerprinting sulfur speciation in aprotic electrolytes is a key to understand fundamental chemistry and design well-performing lithium-sulfur(Li-S)batteries.Lithium polysulfide(LiPS)dissolution and deposition in ether-based electrolytes during redox reactions have been probed and established by spectroscopy and microscopy.However,detailed LiPS structure and solvation properties influenced by conventional and newly developed electrolytes remain elusive,which exert fundamental challenges and practical difficulties in decoupling battery performance from electrolyte volume.This perspective aims to provide timely information to uncover underlying mechanisms that rein in sulfur speciation by considering the charge density of LiPSs and the coordination strength of solvents/salts.The discussion starts with unlocking the baseline electrolyte formulation to investigate its role in LiPS formation and compatibility.After that,the term coordination strength is used instead of donor number and dielectric constant to describe interactions between solvents and LiPSs and to reveal LiPS structure evolution.This work is expected to encourage the discovery of new electrolyte working mechanisms to develop energy-dense and power-intensive Li-S batteries.
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    A regularization algorithm of dynamic light scattering for estimating the particle size distribution of dual-substance mixture in water

    Yanghong WangZiqiang MengZipei ZhangMin Xia...
    246-257页
    查看更多>>摘要：Dynamic light scattering(DLS)is a nondestructive,well-established technique for the size character-ization of proteins,nanoparticles,polymers,and colloidal dispersions.However,current DLS techniques are only applied to particle groups of single composition due to the limitation of their inversion algo-rithm.In this study,we propose a particle size distribution inversion algorithm based on the Tikhnonov regularization method that can be applied to the dual-substance particle mixture.The algorithm re-trieves the particle size distributions of two substances,respectively,by taking advantage of their refractive index differences.The simulation results reveal that the algorithm has excellent accuracy and stability when the scattering angle is 30°.Instead of the original identity matrix,the first-order difference matrix and second-order difference matrix are used as the regular matrix when utilizing the Tikhnonov algorithm,which obviously improves the anti-interference,accuracy,and stability of the algorithm.Furthermore,the inversion of particle size distribution is carried out at a 0.01％-1％noise level,which shows that the algorithm has an available antinoise ability.Finally,experimental particle size mea-surements for a mixture of polystyrene beads and toner particles demonstrate that the proposed algo-rithm is superior to the traditional Tikhnonov algorithm in applicability and accuracy.
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    Optimization of product characteristics of porous carbon agglomerates using a design of experiments in fluidized bed agglomeration

    Martin OelofseRobert RackMarcelle HildenPeter Langguth...
    258-269页
    查看更多>>摘要：Spraying parameters during particle agglomeration processes can affect the agglomeration kinetics and particle growth.This study was conducted to better understand the influence of the spraying parameters in a fluidized bed wet agglomeration process,and the influence on the stability characteristics of carbon tablets.A formulation based on fine carbon and peroxide powder,as well as carboxymethyl cellulose as a binder,was used to produce agglomerates in a first production step.Thereafter in a second production step carbon tablets with a high porosity were molded for the customer goods industry.The optimization of the compressive strength of these carbon tablets was the goal of the trials.Carbon agglomerates were produced with a laboratory scale granulator called"ProCell"and were compressed with a five-cavity mechanical press.The screening of the agglomeration process parameters and their influence on the agglomerates quality,as well as the performance characteristics of the carbon tablets,were investigated using a multilevel factorial design.The experimental runs were done by varying atomized air pressure and feed rate of the fluid.This was determined by the design model.The findings of the statistical trials showed that low atomized air pressure and a low feed rate lead to a higher tablet compressive strength.
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    CFD-DEM study on the synergistic effect of coke consumption and particle dynamics in the blast furnace raceway

    Peng XuPeng HanZhijun HeXizhong An...
    270-278页
    查看更多>>摘要：In this study,the gas-solid flow process in the blast furnace raceway is numerically simulated using coupled computational fluid dynamics and the discrete element method(CFD-DEM).The coke reaction kinetics data are imported into the DEM model to reproduce the consumption process of each coke particle.The effects of inlet gas velocity and angle on the morphology of the raceway,coke consumption rate,coke bed temperature,and particle size distribution in the blast process are systematically inves-tigated and analyzed.The results show that the consumption of coke particles promotes the formation of raceways during the blast process.At the same time,a coke mixture layer is produced at the edge of the raceway.The higher the inlet gas velocity,the thicker the coke mixture layer in the middle and upper parts of the raceway region,and the larger the proportion of small particles in the coke mixture layer.The effect of the inlet gas angle on the raceway region is less than the inlet gas velocity.However,with the increase in the inlet gas angle,the high-temperature region of the coke bed extends downward gradually,which is conducive to activating the hearth.
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