首页|The synergetic enhancement of piezo catalytic performance to remove tetracycline by K2Ti6O13/TiO2 composite

The synergetic enhancement of piezo catalytic performance to remove tetracycline by K2Ti6O13/TiO2 composite

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Piezo catalysis has recently been considered an important technology in environmental treatment. In this study, a type II heterojunction of K2Ti6O13/TiO2 composite is successfully prepared by a hydrothermal method for the highly efficient piezo catalytic degradation of tetracycline. The factors influencing the piezo catalysis of tetracycline are systematically studied and discussed, including pH value, competition of anions/cations, ultrasonic power, ultrasonic frequency, and temperature, etc. Free radical sacrificial agents (EDTA-2Na, DMSO, AgNO3, and P-BQ, etc.) are utilized to better understand the degradation mechanism by piezo catalysis, and holes are found to play a dominant role in the catalytic process, and ·O2- comes the second. The combination of K2Ti6O13 and TiO2 constructs a type II heterojunction of the highly efficient separation of piezo electrons and holes, thus systematically increasing the piezo catalytic performance. This work provides a new idea to degrade organic pollution through piezo catalysis and the potential application of piezo catalysis in environmental treatment.

CompositeK2Ti6O13Piezo catalysisTetracyclineTiO2

Zhang S.、Gao F.、Fang M.、Zhang Y.、Cai Y.、Tan X.、Li K.、Kong M.、Liu H.

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College of Environmental Science and Engineering North China Electric Power University

Key Laboratory of Salt Lake Resources and Chemistry Qinghai Institute of Salt Lakes Chinese Academy of Sciences

Key Laboratory of Materials Physics Institute of Solid State Physics HFIPS Chinese Academy of Sciences

2022

Journal of Alloys and Compounds

Journal of Alloys and Compounds

EISCI
ISSN:0925-8388
年,卷(期):2022.900
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