中国化学工程学报(英文版)2024,Vol.67Issue(3) :126-134.DOI:10.1016/j.cjche.2023.09.016

Enhanced gas production and CO2 storage in hydrate-bearing sediments via pre-depressurization and rapid CO2 injection

Hongnan Chen Yifei Sun Bojian Cao Minglong Wang Ming Wang Jinrong Zhong Changyu Sun Guangjin Chen
中国化学工程学报(英文版)2024,Vol.67Issue(3) :126-134.DOI:10.1016/j.cjche.2023.09.016

Enhanced gas production and CO2 storage in hydrate-bearing sediments via pre-depressurization and rapid CO2 injection

Hongnan Chen 1Yifei Sun 1Bojian Cao 1Minglong Wang 1Ming Wang 1Jinrong Zhong 2Changyu Sun 1Guangjin Chen1
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作者信息

  • 1. State Key Laboratory of Heavy Oil Processing,China University of Petroleum,Beijing 102249,China
  • 2. School of Chemistry and Chemical Engineering,Changsha University of Science & Technology,Changsha 410114,China
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Abstract

Carbon emission reduction and clean energy development are urgent demands for mankind in the coming decades.Exploring an efficient CO2 storage method can significantly reduce CO2 emissions in the short term.In this study,we attempted to construct sediment samples with different residual CH4 hy-drate amounts and reservoir conditions,and then investigate the potentials of both CO2 storage and enhanced CH4 recovery in depleted gas hydrate deposits in the permafrost and ocean zones,respectively.The results demonstrate that CO2 hydrate formation rate can be significantly improved due to the presence of residual hydrate seeds;However,excessive residual hydrates in turn lead to the decrease in CO2 storage efficiency.Affected by the T-P conditions of the reservoir,the storage amount of liquid CO2 can reach 8 times that of gaseous CO2,and CO2 stored in hydrate form reaches 2-4 times.Additionally,we noticed two other advantages of this method.One is that CO2 injection can enhance CH4 recovery rate and increases CH4 recovery by 10%-20%.The second is that hydrate saturation in the reservoir can be restored to 20%-40%,which means that the solid volume of the reservoir avoids serious shrinkage.Obviously,this is crucial for protecting the goaf stability.In summary,this approach is greatly promising for high-efficient CO2 storage and safe exploitation of gas hydrate.

Key words

Hydrate/Depressurization/CO2 storage/CH4 production/Reservoir remediation

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基金项目

国家自然科学基金(22378424)

国家自然科学基金(52004136)

国家自然科学基金(22127812)

国家自然科学基金(U20B6005)

Science Foundation of China University of Petroleum Beijing(2462023BJRC017)

Hunan Provincial Department of Education Scientific Research Project(22B0310)

出版年

2024
中国化学工程学报(英文版)
中国化工学会

中国化学工程学报(英文版)

CSTPCDEI
影响因子:0.818
ISSN:1004-9541
参考文献量38
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