首页|Aggregation-regulated bioreduction process of graphene oxide by Shewanella bacteria

Aggregation-regulated bioreduction process of graphene oxide by Shewanella bacteria

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The bioreduction of graphene oxide(GO)using environmentally functional bacteria such as Shewanella represents a green approach to produce reduced graphene oxide(rGO).This process differs from the chemical reduction that involves instantaneous molecular reactions.In bioreduction,the contact of bacterial cells and GO is considered the rate-limiting step.To reveal how the bacteria-GO integration regulates rGO production,the comparative experiments of GO and three Shewanella strains were carried out.Fourier-transform infrared spectroscopy,X-ray photoelectron spectroscopy,Raman spectroscopy,and atomic force microscopy were used to characterize the reduction degree and the aggregation degree.The results showed that a spontaneous aggregation of GO and Shewanella into the condensed entity occurred within 36 h.A positive linear correlation was established,linking three indexes of the aggre-gation potential,the bacterial reduction ability,and the reduction degree(ID/IG)comprehensively.

Graphene oxideReduced graphene oxideBioreductionAggregationShewanella

Kaixin Han、Yibo Zeng、Yinghua Lu、Ping Zeng、Liang Shen

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Department of Chemical and Biochemical Engineering,College of Chemistry and Chemical Engineering,Xiamen University,Xiamen 361005,China

Pen-Tung Sah Institute of Micro-Nano Science and Technology,Xiamen University,Xiamen 361005,China

Chinese Research Academy of Environmental Sciences,Beijing 100012,China

National Natural Science Foundation of ChinaNatural Science Foundation of Fujian Province of China

221782932022J01022

2024

中国化学工程学报(英文版)
中国化工学会

中国化学工程学报(英文版)

CSTPCDEI
影响因子:0.818
ISSN:1004-9541
年,卷(期):2024.69(5)