首页|Process synthesis for the separation of coal-to-ethanol products

Process synthesis for the separation of coal-to-ethanol products

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The coal-to-ethanol process,as the clean coal utilization,faces challenges from the energy-intensive distillation that separates multi-component effluents for pure ethanol.Referring to at least eight col-umns,the synthesis of the ethanol distillation system is impracticable for exhaustive comparison and difficult for conventional superstructure-based optimization as rigorous models are used.This work adopts a superstructure-based framework,which combines the strategy that adaptively selects branches of the state-equipment network and the parallel stochastic algorithm for process synthesis.High-performance computing significantly reduces time consumption,and the adaptive strategy substan-tially lowers the complexity of the superstructure model.Moreover,parallel computing,elite search,population redistribution,and retention strategies for irrelevant parameters are used to improve the optimization efficiency further.The optimization terminates after 3000 generations,providing a flow-sheet solution that applies two non-sharp splitting options in its distillation sequence.As a result,the 59-dimension superstructure-based optimization was solved efficiently via a differential evolution al-gorithm,and a high-quality solution with a 28.34%lower total annual cost than the benchmark was obtained.Meanwhile,the solution of the superstructure-based optimization is comparable to that ob-tained by optimizing a single specific configuration one by one.It indicates that the superstructure-based optimization that combines the adaptive strategy can be a promising approach to handling the process synthesis of large-scale and complex chemical processes.

Coal-to-ethanolProcess synthesisSuperstructure-based optimizationDifferential evolution algorithmDistillation

Qingping Qu、Daoyan Liu、Hao Lyu、Jinsheng Sun

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School of Chemical Engineering and Technology,Tianjin University,Tianjin 300072,China

Sustainable Energy and Environment Thrust,The Hong Kong University of Science and Technology(Guangzhou),Nansha 511400,China

2024

中国化学工程学报(英文版)
中国化工学会

中国化学工程学报(英文版)

CSTPCDEI
影响因子:0.818
ISSN:1004-9541
年,卷(期):2024.69(5)
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