中国化学工程学报(英文版)2024,Vol.71Issue(7) :140-147.DOI:10.1016/j.cjche.2024.03.024

Four-channel catalytic micro-reactor based on alumina hollow fiber membrane for efficient catalytic oxidation of CO

Baichuan Xu Bin Wang Tao Li
中国化学工程学报(英文版)2024,Vol.71Issue(7) :140-147.DOI:10.1016/j.cjche.2024.03.024

Four-channel catalytic micro-reactor based on alumina hollow fiber membrane for efficient catalytic oxidation of CO

Baichuan Xu 1Bin Wang 1Tao Li1
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作者信息

  • 1. Key Laboratory of Energy Thermal Conversion and Control of Ministry of Education,School of Energy and Environment,Southeast University,Nanjing 211100,China
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Abstract

The traditional automotive catalytic converter using commercial ceramic honeycomb carriers has many problems such as high back pressure,low engine efficiency,and high usage of precious metals. This study proposes a four-channel catalytic micro-reactor based on alumina hollow fiber membrane,which uses phase inversion method for structural molding and regulation. Due to the advantages of its carrier,it can achieve lower ignition temperature under low noble metal loading. With Pd/CeO2 at a loading rate of 2.3%(mass),the result showed that the reaction ignition temperature is even less than 160 ℃,which is more than 90 ℃ lower than the data of commercial ceramic substrates under similar catalyst loading and airspeed conditions. The technology in turn significantly reduces the energy consumption of the reaction. And stability tests were conducted under constant conditions for 1000 h,which proved that this catalytic converter has high catalytic efficiency and stability,providing prospects for the design of innovative catalytic converters in the future.

Key words

Catalytic converter/Precious metal catalyst/Phase inversion method/Hollow fiber membrane/CO oxidation

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基金项目

Natural Science Foundation of Jiangsu Province(BK20210252)

出版年

2024
中国化学工程学报(英文版)
中国化工学会

中国化学工程学报(英文版)

CSTPCDEI
影响因子:0.818
ISSN:1004-9541
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