首页|Open-Shell Oligomers and Polymers:Theory,Characterization Methods,Molecular Design,and Applications
Open-Shell Oligomers and Polymers:Theory,Characterization Methods,Molecular Design,and Applications
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Open-shell oligomers and polymers have exhibited intriguing electronic and magnetic properties,making them highly desirable for a wide range of applications,including ambipolar organic field-effect transistors(OFETs),photodetectors,organic thermoelectrics,and spintronics.Although open-shell ground states have been observed in certain small molecules and doped organic semiconductors,the exploration of open-shell ground-state conjugated polymers is still limited,and the strategies for designing these polymers remain obscure.This review aims to briefly introduce the theory and characterization methods of open-shell conjugated polymers,along with an overview of recent progress and applica-tions.The objective is to stimulate further advancements and investigations in this promising area by shedding light on the potential of open-shell conjugated polymers and the challenges that lie ahead.
Conjugated polymersOpen-shell moleculesHigh-spin ground stateDonor-acceptor(D-A)polymersOptoelectronic and magnetic properties
Xue-Qing Wang、Cheng Song、Ting Lei
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Key Laboratory of Polymer Chemistry and Physics(Ministry of Education),School of Materials Science and Engineering,Peking University,Beijing 100871,China
北京市自然科学基金King Abdullah University of Science and Technology Research Funding(KRF)
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