材料科学技术(英文版)2021,Vol.95Issue(36) :203-212.

Controlled multilevel switching and artificial synapse characteristics in transparent HfAlO-alloy based memristor with embedded TaN nanoparticles

Chandreswar Mahata Hassan Algadi Muhammad Ismail Daewoong Kwon Sungjun Kim
材料科学技术(英文版)2021,Vol.95Issue(36) :203-212.

Controlled multilevel switching and artificial synapse characteristics in transparent HfAlO-alloy based memristor with embedded TaN nanoparticles

Chandreswar Mahata 1Hassan Algadi 2Muhammad Ismail 1Daewoong Kwon 3Sungjun Kim1
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作者信息

  • 1. Division of Electronics and Electrical Engineering,Dongguk University,Seoul 04620,Republic of Korea
  • 2. Department of Electrical Engineering,Faculty of Engineering,Najran University,P.O.Box 1988,Najran 11001,Saudi Arabia
  • 3. Department of Electrical Engineering,Inha University,Incheon,Republic of Korea
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Abstract

Atomic layer deposition technique has been used to prepare tantalum nitride nanoparticles (TaN-NPs)and sandwiched between Al-doped HfO2 layers to achieve ITO/HfAlO/TaN-NP/HfAlO/ITO RRAM device.Transmission electron microscopy along with energy dispersive spectroscopy confirms the presence of TaN-NPs.X-ray photoelectron spectroscopy suggests that part of TaN converted to tantalum oxynitride(TaOxNy) which plays an important role in stable cycle-to-cycle resistive switching.Charge trapping and oxygen vacancy creation were found to be modified after the inclusion of TaN-NPs inside RRAM struc-ture.Also,HfAlO/TaOxNy interface due to the presence TaN-NPs improves the device-to-device switching reliability by reducing the probability of random rupture/formation of conductive filaments (CFs).DC en-durance of more than 103 cycles and memory data retention up to 104 s was achieved with an insignif-icant variation of different resistance states.Multilevel conductance was attained by controlling RESET voltage with stable data retention in multiple states.The volatile threshold switching was monitored af-ter controlling the CF forming at 200 nA current compliance with high selectivity of~103.Synaptic learn-ing behavior has been demonstrated by spike-rate-dependent plasticity (SRDP).Reliable potentiation and depression processes were observed after the application of suitable negative and positive pulses which shows the capability of the TaN-NPs based RRAM device for transparent synaptic devices.

Key words

RRAM/ALD TaN-nanoparticles/Threshold switching/Spike-rate-dependent plasticity/Multilevel conductance/Synaptic properties

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基金项目

National Research Foundation of Korea (NRF) grant funded by the Korean gov-ernment (MSIP)(2018R1C1B5046454)

Dongguk University Research Fund of 2020(2018R1C1B5046454)

Dongguk University Research Fund of 2020()

出版年

2021
材料科学技术(英文版)
中国金属学会 中国材料研究学会 中国科学院金属研究所

材料科学技术(英文版)

CSTPCDCSCDSCI
影响因子:0.657
ISSN:1005-0302
参考文献量64
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