材料科学技术(英文版)2022,Vol.99Issue(4) :55-60.

Mictomagnetism and suppressed thermal conduction of the prototype high-entropy alloy CrMnFeCoNi

Jianyan Yang Weijun Ren Xinguo Zhao Tatsuya Kikuchi Ping Miao Kenji Nakajima Bing Li Zhidong Zhang
材料科学技术(英文版)2022,Vol.99Issue(4) :55-60.

Mictomagnetism and suppressed thermal conduction of the prototype high-entropy alloy CrMnFeCoNi

Jianyan Yang 1Weijun Ren 2Xinguo Zhao 2Tatsuya Kikuchi 3Ping Miao 4Kenji Nakajima 3Bing Li 1Zhidong Zhang1
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作者信息

  • 1. Shenyang National Laboratory for Materials Science,Institute of Metal Research,Chinese Academy of Sciences,Shenyang 110016,China;School of Materials Science and Engineering,University of Science and Technology of China,Shenyang 110016,China
  • 2. Shenyang National Laboratory for Materials Science,Institute of Metal Research,Chinese Academy of Sciences,Shenyang 110016,China
  • 3. J-PARC Center,Japan Atomic Energy Agency,Tokai 319-1112,Ibaraki,Japan
  • 4. Institute of Materials Structure Science,High Energy Accelerator Research Organization(KEK),Tokai 319-1106,Ibaraki,Japan;Institute of High Energy Physics,Chinese Academy of Sciences,Beijing 100049,China;China Spallation Neutron Source Science Center,Dongguan 523803,Guangdong,China
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Abstract

High-entropy alloys are characteristic of extensive atomic occupational disorder on high-symmetric lat-tices,differing from traditional alloys.Here,we investigate the magnetic and thermal transport proper-ties of the prototype face-centered-cubic high-entropy alloy CrMnFeCoNi by combining physical proper-ties measurements and neutron scattering.Direct-current and alternating-current magnetizations mea-surements indicate a mictomagnetic behavior with coexisting antiferromagnetic and ferromagnetic in-teractions below room temperature and three anomalies are found at about 80,40,and 20 K,which are related to the paramagnetic to antiferromagnetic transition,the antiferromagnetic to ferromagnetic transition,and the spin freezing,respectively.The electrical and thermal conductivities are significantly reduced compared to Ni,and the temperature dependence of lattice thermal conductivity exhibits a glass-like plateau.Inelastic neutron scattering measurements suggest weak anharmonicity so that the thermal transport is expected to be dominated by the defect scattering.

Key words

High-entropy alloys/Magnetism/Inelastic neutron scattering/Lattice dynamics/Thermal conductivity

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基金项目

Liaoning Revital-ization Talents Program(XLYC1807122)

National Natu-ral Science Foundation of China(11804346)

National Natu-ral Science Foundation of China(12005243)

National Natu-ral Science Foundation of China(51771197)

Key Research Program of Frontier Sciences of Chi-nese Academy of Sciences(ZDBS-LY-JSC002)

Ministry of Science and Technology of China(2020YFA0406002)

beam time provided by J-PARC through proposal(2018A0176)

出版年

2022
材料科学技术(英文版)
中国金属学会 中国材料研究学会 中国科学院金属研究所

材料科学技术(英文版)

CSTPCDCSCDSCI
影响因子:0.657
ISSN:1005-0302
参考文献量38
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