首页|In situ study on the oscillation of mobile droplets and force analysis during the directional solidification of Al-Bi alloy

In situ study on the oscillation of mobile droplets and force analysis during the directional solidification of Al-Bi alloy

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During solidifications of immiscible alloys,the motion of droplets at the solid/liquid(S/L)interface is gen-erally driven by dragging force,gravity force,repulsion force of interface,and thermal-solutal Marangoni force,However,there is few in situ study investigating kinetics behavior to analyze the forces on droplets.The mechanism of droplet motion remains unclear due to the unavailability or uncertainty of the effect of convection and solutal Marangoni force on droplet behavior.In this study,directional solidification of im-miscible Al-Bi alloy was observed via synchrotron radiography,and the horizontal oscillation of droplets at S/L interface was detected for the first time.Forces,especially solutal Marangoni force,were calcu-lated based on the in situ measured radius of droplets and thermal-solutal gradients.The experimental results cannot be reasonably explained by the previous analysis model which neglects melt convection.The non-negligible effect of flow on droplet motion was demonstrated,and the force balance of droplet both vertically and horizontally can be obtained considering a lift force of 6.39 × 10-9 N and a modified solute-related parameter dσ/dc of 0.45-0.65 J m-2,respectively.

RadiographySolidificationImmiscible alloysDroplet behaviorSolid/liquid interface

Ya Zhang、Yue Wu、Yang Tang、Jianbo Ma、Bo Mao、Yanling Xue、Hui Xing、Jiao Zhang、Baode Sun

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Shanghai Key Lab of Advanced High-temperature Materials and Precision Forming and State Key Lab of Metal Matrix Composites,Shanghai Jiao Tong University, Shanghai 200240,China

Shanghai Synchrotron Radiation Facility,Shanghai Advanced Research Institute,CAS,Shanghai 201204,China

Collaborative Innovation Center for Advanced Ship and Deep-sea Exploration,Shanghai Jiao Tong University,Shanghai 200240,China

National Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaShanghai Pujiang ProgramUSAX beamline at Shanghai Synchrotron Radiation Facility(SSRF)

522710365197123721PJD030

2024

材料科学技术(英文版)
中国金属学会 中国材料研究学会 中国科学院金属研究所

材料科学技术(英文版)

CSTPCD
影响因子:0.657
ISSN:1005-0302
年,卷(期):2024.177(10)
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