材料科学技术(英文版)2024,Vol.178Issue(11) :22-28.DOI:10.1016/j.jmst.2023.08.044

Construction of one-dimensional hierarchical MoS2/Ni3S2 composites with enhanced interfacial polarization and improved wideband microwave absorption

Kaicheng Luo Biao Zhao Chunyang Xu Chongyun Liang Chang Zhang Yiqian Du Xiaowei Lv Jincang Zhang Limin Wu Renchao Che
材料科学技术(英文版)2024,Vol.178Issue(11) :22-28.DOI:10.1016/j.jmst.2023.08.044

Construction of one-dimensional hierarchical MoS2/Ni3S2 composites with enhanced interfacial polarization and improved wideband microwave absorption

Kaicheng Luo 1Biao Zhao 2Chunyang Xu 1Chongyun Liang 1Chang Zhang 3Yiqian Du 1Xiaowei Lv 1Jincang Zhang 3Limin Wu 4Renchao Che5
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作者信息

  • 1. Laboratory of Advanced Materials,Shanghai Key Lab of Molecular Catalysis and Innovative Materials,Academy for Engineering & Technology,Fudan University,Shanghai,200438,China
  • 2. School of Microelectronics.Fudan University,Shanghai,200433,China
  • 3. Zhejiang Laboratory,Hangzhou,311100,China
  • 4. Inner Mongolia University,Hohhot,010021,China
  • 5. Laboratory of Advanced Materials,Shanghai Key Lab of Molecular Catalysis and Innovative Materials,Academy for Engineering & Technology,Fudan University,Shanghai,200438,China;Zhejiang Laboratory,Hangzhou,311100,China
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Abstract

The construction of one-dimensional(1D)sulfides has attracted extensive attention for improving mi-crowave absorption(MA)performance owing to the anisotropic conductive networks.However,the syn-thesis of conductive 1D hierarchical materials with unique interfacial polarization and excellent MA prop-erties remains challenging.In this study,cable-like MoS2/Ni3S2 was synthesized by a one-step hydrother-mal strategy.The complex permittivity of the binary composites could be improved by tuning the thick-ness of the MoS2 coating.Importantly,the construction of heterogeneous contacts by MoS2 and Ni3S2 contributed to enhanced polarization loss,and the charge distribution was validated by electron holog-raphy.The wide efficient absorption bandwidth can reach above 4.8 GHz at a thin thickness.These new discoveries shed light on novel structures for 1D sulfide materials and the design of functional core-shell composites for microwave absorption.

Key words

1D sulfide materials/Microwave absorption/MoS2/Ni3S2/Interfacial polarization/Core-shell composites

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基金项目

Ministry of Science and Technology of China(2021YFA1200600)

Ministry of Science and Technology of China(2018YFA0209100)

National Natural Science Foundation of China(52231007)

National Natural Science Foundation of China(51725101)

National Natural Science Foundation of China(11727807)

出版年

2024
材料科学技术(英文版)
中国金属学会 中国材料研究学会 中国科学院金属研究所

材料科学技术(英文版)

CSTPCDCSCD
影响因子:0.657
ISSN:1005-0302
参考文献量41
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