材料科学技术(英文版)2024,Vol.198Issue(31) :1-11.DOI:10.1016/j.jmst.2024.01.063

Biochar decorated Bi4O5Br2/g-C3N4 S-scheme heterojunction with enhanced photocatalytic activity for Norfloxacin degradation

Chao Chen Xiaofei Zhang Enzhou Liu Jingsan Xu Jing Sun Huanxian Shi
材料科学技术(英文版)2024,Vol.198Issue(31) :1-11.DOI:10.1016/j.jmst.2024.01.063

Biochar decorated Bi4O5Br2/g-C3N4 S-scheme heterojunction with enhanced photocatalytic activity for Norfloxacin degradation

Chao Chen 1Xiaofei Zhang 1Enzhou Liu 2Jingsan Xu 3Jing Sun 1Huanxian Shi1
扫码查看

作者信息

  • 1. School of Pharmacy,Shaanxi Province Key Laboratory of New Drugs and Chinese Medicine,Shaanxi University of Chinese Medicine,Xianyang 712046,China
  • 2. School of Chemical Engineering/Xi'an Key Laboratory of Special Energy Materials,Northwest University,Xi'an 710069,China
  • 3. School of Chemistry and Physics,Queensland University of Technology,Brisbane,QLD 4000,Australia
  • 折叠

Abstract

In this work,a novel biochar decorated Bi4O5Br2/g-C3N4 S-scheme heterojunction was successfully pre-pared for Norfloxacin(NOR)degradation,and it was found that the 5%-Bi4O5Br2/g-C3N4/C heterojunction exhibited the excellent photocatalytic degradation activity toward NOR,degrading 92.5%of NOR within 72 min under visible light irradiation.The effects of pH,dosage,and concentration of the NOR on the photocatalytic activity were also systematically investigated.The mechanism studies revealed that the active species like hole(h+),hydroxyl radical(·OH),and superoxide radical(·O2-)play a predominant role in the NOR degradation,and the enhanced removal rate of Bi4O5Br2/g-C3N4/C heterojunction can be attributed to the synergistic effect of adsorption and photocatalytic process.In addition,an S-scheme transfer channel in the interface of the Bi4O5Br2/g-C3N4/C heterojunction is proposed,which can effec-tively improve the separation of the photogenerated carriers and enhance the photocatalytic performance.This research provides inspiration for designing S-scheme heterojunction for wastewater treatment.

Key words

S-scheme heterojunction/g-C3N4/Biochar/Photocatalytic degradation/Norfloxacin

引用本文复制引用

出版年

2024
材料科学技术(英文版)
中国金属学会 中国材料研究学会 中国科学院金属研究所

材料科学技术(英文版)

CSTPCDCSCD
影响因子:0.657
ISSN:1005-0302
段落导航相关论文