首页|2020年宣城市臭氧污染特征及气象影响因素分析

2020年宣城市臭氧污染特征及气象影响因素分析

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基于宣城市2020年环境空气质量监测数据及同期气象观测数据分析了臭氧(O3)污染特征和气象成因.结果表明:2020年臭氧日最大滑动8小时平均质量浓度第90百分位数(MDA8-90)为137μg/m3,相对2019年增长了2.2%.MDA8-90的月变化趋势呈"M"型,峰值出现在9月(164μg/m3).O3小时浓度日变化呈单峰型,峰值出现在16时,谷值出现在7时.不同天气条件下,晴天O3质量浓度峰值最高,多云、阴天和雨天的O3浓度峰值依次递减.O3质量浓度与气温呈现正相关性,与相对湿度和NO2质量浓度呈现显著的负相关性.气温大于25℃、相对湿度小于50%及风速低于2 m/s的气象条件与高质量浓度O3污染密切相关.进而利用潜在源贡献函数模型分析了污染传输对宣城市O3质量浓度的影响及潜在传输源区分布特征,结果表明不同时期O3潜在来源差异明显,6―8月的主要潜在来源位于东海海面和浙江北部区域,而9―11月的分布在苏皖豫鲁交界处和赣鄂交界处.
Characteristics of surface ozone pollution and meteorological parameters analysis in Xuancheng City in 2020
The characteristics and meteorological causes of ozone (O3) pollution in Xuancheng City,China,were analyzed based on the ambient air quality monitoring data in 2020 and the meteorological observation data of the same period. The results indicated that the 90th percentile of the maximum daily sliding 8-hour average mass concentration of O3 (MDA8-90) in 2020 was 137 μg/m3,with an increase of 2.2% compared to 2019. The monthly variation of MDA8-90 showed an "M" type,with the peak appearing in September (164 μg/m3). The diurnal variation showed a unimodal pattern,with the peak at 16:00 and the trough at 07:00. Under different weather conditions,the peak value of O3 mass concentration was the highest on sunny days,and decreased sequentially on cloudy,overcast sky and rainy days. O3 mass concentration revealed a positive correlation with temperature and a significant negative correlation with relative humidity and NO2 concentration. Specifically,meteorological conditions with air temperatures>25 ℃,relative humidity<50%,and a wind speed<2 m/s were closely related to high concentrations of O3. In addition,the potential source contribution function model (PSCF) was used to analyze the impact of pollution transport on the O3 mass concentration in Xuancheng and the distribution characteristics of potential transport sources. The results showed that the potential sources of O3 at different stages were significantly different in various periods of the year. The main potential sources of O3 from June to August were distributed in the East China Sea and the northern part of Zhejiang Province,while the main potential sources of O3 from September to November were distributed at the junction of Jiangsu,Anhui,Henan and Shandong,as well as the junction of Jiangxi and Hubei Province.

Xuancheng Cityozonevariation characteristicmeteorological factorspotential source analysis function

姚笛、陈浩、王明、张帅、刘东

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宣城市生态环境局,安徽 宣城 242099

合肥中科光博量子科技有限公司,安徽 合肥 230088

中国科学院合肥物质科学研究院安徽光学精密机械研究所,中国科学院大气光学重点实验室,安徽合肥 230031

宣城市 臭氧 变化特征 气象因素 潜在源区

2024

大气与环境光学学报
中国科学院安徽光学精密机械研究所

大气与环境光学学报

影响因子:0.285
ISSN:1673-6141
年,卷(期):2024.19(5)