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西南喀斯特地区水体溶解无机碳时空分布特征及其来源分析

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碳循环是地球主要物质循环之一,对全球气候变化与人类发展具有重要影响.本文梳理了近年来嘉陵江水系、乌江水系、赤水河水系及西江水系溶解无机碳的相关研究成果,对西南喀斯特地区水体溶解无机碳(DIC)与碳同位素(13δCDIC)的时空分布特征、影响因素及其来源进行全域性视角分析,并得出以下结论:(1)西南喀斯特地区水体DIC含量与δ13CDIC值在各水系之间存在差异性,具有显著时空分布特征,其中赤水河水系DIC含量(2.79mmol/L)与δ13CDIC值(-8.15‰)均最高,西江水系DIC含量(1.95 mmol/L)与δ13CDIC值(-10.6‰)最低;(2)该地区DIC含量变化受到碳酸盐岩化学风化、气候变化及人类活动等因素的综合影响;(3)流域内DIC主要来源于碳酸盐岩风化与土壤CO2.研究结果有助于推动河流流域溶解无机碳变化的研究,为我国水体碳循环研究提供理论基础.
Spatial-temporal Distribution and Sources of Dissolved Inorganic Carbon in Karst Water,Southwest China
The carbon cycle constitutes one of the major occurring material cycles,with a large influence on human development and global climate change.This paper reviews recent research on dissolved inorganic carbon(DIC)in the Jialing River basin,Wujiang River basin,Chishui River basin,and Xijiang River basin.It provides a comprehensive analysis from a regional perspective on the spatiotemporal distribution,influencing factors,and sources of DIC and carbon isotopes(δ13CDIC)in the water bodies of the southwestern karst region.The conclusions are as follows:(1)There were variations in DIC concentration and δ13CDIC values among the different water systems,with notable spatiotemporal distribution.The Chishui River basin exhibited the highest DIC concentration(2.79 mmol/L)and δ13CDIC value(-8.15‰),while the Xijiang River basin had the lowest DIC concentration(1.95 mmol/L)and δ13CDIC value(-10.6‰).(2)DIC concentration changes in the region were influenced by a combination of factors,including carbonate rock chemical weathering,climate change,and human activities.(3)DIC in the watershed is primarily derived from carbonate rock weathering and soil CO2.These research results contribute to advancing the study of DIC variations in river basins and provide a theoretical foundation for carbon cycling in water bodies in China.

southwest karst regiondissolved inorganic carbonstable carbon isotopesspatial and temporal distributioninfluencing factors

张晓慧、焦树林、杨柳英、韦宗校、张文龙

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贵州师范大学地理与环境科学学院/喀斯特研究院,贵阳 550025

贵州省喀斯特山地生态环境国家重点实验室培育基地,贵阳 550025

西南喀斯特地区 溶解无机碳 稳定碳同位素 时空分布 影响因素

贵州省科技支撑项目

黔科合支撑[2023]一般214

2024

地球与环境
中国科学院地球化学研究所

地球与环境

CSTPCD北大核心
影响因子:0.875
ISSN:1672-9250
年,卷(期):2024.52(5)