首页|共代谢降解感潮河道底泥多环芳烃的效能研究

共代谢降解感潮河道底泥多环芳烃的效能研究

扫码查看
感潮河道由于受潮汐影响,上覆水盐度波动大且区域差异明显,因此,在应用微生物共代谢降解感潮河道底泥中多环芳烃(polycyclic aromatic hydrocarbons,PAHs)时,考察不同盐度对PAHs降解的影响具有一定的实际意义.本研究采用乙酸钠耦合邻苯二甲酸为共代谢底物,考察上覆水0‰~40‰盐度范围对PAHs降解,底泥理化性质(pH,ORP)及底泥硫代谢(酸可挥发性硫化物(acid volatile sulfide,AVS),SO42-)的影响.研究结果表明:在上覆水盐度波动从10‰增大到 50‰时,底泥PAHs降解存在较大差异,低盐环境更利于PAHs的降解,高盐度上覆水易导致微生物共代谢过程中底泥AVS和SO42-的富集.本研究探讨了感潮河道盐度对生物共代谢法降解底泥PAHs污染效能的影响,为感潮河道不同盐度波动条件下底泥难降解有机物去除研究提供理论基础.
Study on the Efficacy of Co-metabolism in Degrading Polycyclic Aromatic Hydrocarbons in Tidal River Sediments
Due to the tidal influence of tidal rivers,the salinity of the overlying water fluctuates greatly and has significant regional differences.Therefore,it is of practical importance to investigate the effects of different salinity on the degradation of polycyclic aromatic hydrocarbons(PAHs)in the sediment of tidal rivers when applying microbial co-metabolism.In this study,sodium acetate coupled with phthalic acid was used as the co-metabolizing sediment to investigate the effects of 0‰~40‰salinity of the overlying water on the degradation of PAHs,the physicochemical properties(pH,ORP)and the sulfur metabolism(acid volatile sulfide(AVS),SO42-)of the sediment.The results of the study showed that there were large differences in the degradation of PAHs in the sediment when the salinity fluctuation of the overlying water increased from 10‰to 50‰.The low salinity environment was more favorable for the degradation of PAHs,and the high salinity overlying water was prone to lead to the enrichment of AVS and SO42-in the sediment during the process of microbial co-metabolism.In this study,we investigated the effect of salinity on the degradation efficiency of PAHs pollution in substrate by biological co-metabolism in tidal rivers,and provided a theoretical basis for the study of the removal of difficult organic matter in substrate under different salinity fluctuation conditions in tide-sensitive rivers.

tidal riversediment PAHssalinityco-metabolism

吴阳、王宏杰、李龙、刘杰、李朝祥、王锋

展开 >

深圳市供排水行业协会,广东 深圳 518000

哈尔滨工业大学(深圳)土木与环境工程学院,广东 深圳 518055

城市水资源与水环境国家重点实验室(哈尔滨工业大学),黑龙江 哈尔滨 150090

中山市市政排水事务中心,广东 中山 528400

深圳市万木水务有限公司,广东 深圳 518055

哈尔滨工业大学(深圳)经济管理学院,广东 深圳 518055

展开 >

感潮河道 底泥多环芳烃 盐度 共代谢

深圳市科技创新委员会可持续发展专项

KCXFZ202002011006362

2024

广东化工
广东省石油化工研究院

广东化工

影响因子:0.288
ISSN:1007-1865
年,卷(期):2024.51(19)