首页|乌鲁木齐市区大气氮素干沉降的输入性分析

乌鲁木齐市区大气氮素干沉降的输入性分析

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2009年8月至2010年3月在乌鲁木齐市及城郊,通过大气颗粒物采样器、气体被动采样器对大气氮素干沉降进行连续性监测。结果表明:除NH3浓度值ISFR(土肥所)高于XIEG(生地所)外,其他活性氮成分的浓度XIEG均大于ISFR。NO2-N,NH3-N(气态),PNO 3--N,PNH 4+-N(气溶胶态)和PM10(空气动力学当量直径在10μm以下的颗粒物)在监测点XIEG的平均浓度为4.31,4.49,2.52,11.84,224.66μg/m3,在ISFR的监测值为2.32,4.63,2.34,7.59和188.16μg/m3。根据每月平均浓度值的变化讨论了不同活性氮的时空变异,基于浓度和所引用文献中的沉降速率,得出XIEG大气氮素干沉降的通量为28.68 kg/(hm2.a),ISFR通量为21.60 kg/(hm2.a)。如此高通量中铵态氮占到65.69%(XIEG)和69.44%(ISFR),8~11月以NH3为主,12~3月则主要是气溶胶态NH4+。
Analysis on Input of Atmospheric Nitrogen Dry Deposition in Urumqi
Atmospheric concentrations of NH3,NO2,particulate NH+4(PNH+4) and NO-3(PNO-3) were measured from the samples collected with passive samplers and particulate samplers in Urumqi and its suburbs during the period from August 2009 to March 2010 to estimate atmospheric dry deposition of nitrogen(N) in this region.The results show that NH3 concentration at the Institute of Soil and Fertilizer Research(ISFR,suburban site) was higher than that at the Xinjiang Institute of Ecology and Geography(XIEG,urban site),while the concentrations of other atmospheric reactive N compositions(NO2,particulate NH+4 and NO-3) were higher at XIEG than those at ISFR.The mean concentrations of NH3-N,NO2-N,PNH+4-N,PNO-3-N and PM10(particulate matters with aerodynamic diameter less than 10 μm) at XIEG were 4.49,4.31,2.52,11.84 and 225 μg/m3,and those at ISFR were 4.63,2.32,2.34,7.59 and 188 μg/m3,respectively.Based on the measured concentrations and the dry deposition velocities cited from the references,it was estimated that the atmospheric dry deposition of N was 28.7 kg/(hm2·a) during the sampling period at XIEG and 21.6 kg/(hm2·a) at ISFR,in which the proportion of NHx(NH3+ PNH+4) accounted for 65.7% at XIEG and 69.4% at ISFR,NH3 was dominant during the period from August to November,and PNH+4 was dominant during the period from December to next March.

atmospheric nitrogen depositiondry depositionreactive nitrogenecological effectUrumqi

张伟、刘学军、胡玉昆、李凯辉、沈健林、骆晓声、宋韦

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中国科学院干旱区生物地理与生物资源重点实验室中国科学院新疆生态与地理研究所,新疆乌鲁木齐830011 中国科学院研究生院,北京100049

中国科学院干旱区生物地理与生物资源重点实验室中国科学院新疆生态与地理研究所,新疆乌鲁木齐830011 中国农业大学资源与环境学院,北京100193

中国科学院干旱区生物地理与生物资源重点实验室中国科学院新疆生态与地理研究所,新疆乌鲁木齐830011

中国科学院亚热带农业生态研究所,湖南长沙410125

中国农业大学资源与环境学院,北京100193

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大气氮沉降 干沉降 活性氮 生态效应 乌鲁木齐

中国科学院"百人计划"项目国家重点基础研究发展规划(973计划)

2009CB825103

2011

干旱区研究
中国科学院新疆生态与地理研究所 中国土壤学会

干旱区研究

CSTPCDCSCD北大核心
影响因子:1.157
ISSN:1001-4675
年,卷(期):2011.28(4)
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