Technologies for investigating single-molecule chemical reactions

扫码查看

原文链接

NETL
NSTL
万方数据

外文摘要：Single molecules,the smallest independently stable units in the material world,serve as the fundamental building blocks of matter.Among different branches of single-molecule sciences,single-molecule chemical reactions,by revealing the behavior and properties of individual molecules at the molecular scale,are particularly attractive because they can advance the understanding of chemical reaction mechanisms and help to address key scientific problems in broad fields such as physics,chemistry,biology and materials science.This review provides a timely,comprehensive overview of single-molecule chemical reactions based on various technical platforms such as scanning probe microscopy,single-molecule junction,single-molecule nanostructure,single-molecule fluorescence detection and crossed molecular beam.We present multidimensional analyses of single-molecule chemical reactions,offering new perspectives for research in different areas,such as photocatalysis/electrocatalysis,organic reactions,surface reactions and biological reactions.Finally,we discuss the opportunities and challenges in this thriving field of single-molecule chemical reactions.

外文关键词：

chemical reactionscanning probe microscopysingle-molecule junctionsingle-molecule fluorescencecrossed molecular beam

作者：

Chunyan Gao、Qinghua Gao、Cong Zhao、Yani Huo、Zhizhuo Zhang、Jinlong Yang、Chuancheng Jia、Xuefeng Guo

展开 >

作者单位：

Center of Single-Molecule Sciences,Institute of Modern Optics,Frontiers Science Center for New Organic Matter,Tianjin Key Laboratory of Micro-scale Optical Information Science and Technology,College of Electronic Information and Optical Engineering,Nankai University,Tianjin 300350,China

Hefei National Research Center for Physical Sciences at Microscale,University of Science and Technology of China,Hefei 230026,China

Beijing National Laboratory for Molecular Sciences,National Biomedical Imaging Center,College of Chemistry and Molecular Engineering,Peking University,Beijing 100871,China

基金：

National Key Research and Development Program of ChinaNational Key Research and Development Program of ChinaNational Key Research and Development Program of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNatural Science Foundation of BeijingBeijing National Laboratory for Molecular Sciences

项目编号：

2021YFA12001022021YFA12001012022YFE0128700221730502215001321727806219330012222009BNLMS-CXXM-202407

出版年：

2024

DOI：

10.1093/nsr/nwae236

国家科学评论(英文版)

CSTPCD

ISSN：

年,卷(期)：2024.11(8)