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Spin-dependent electrocatalysis

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The shift towards sustainable energy requires efficient electrochemical conversion technologies,emphasizing the crucial need for robust electrocatalyst design.Recent findings reveal that the efficiency of some electrocatalytic reactions is spin-dependent,with spin configuration dictating performance.Consequently,understanding the spin's role and controlling it in electrocatalysts is important.This review succinctly outlines recent investigations into spin-dependent electrocatalysis,stressing its importance in energy conversion.It begins with an introduction to spin-related features,discusses characterization techniques for identifying spin configurations,and explores strategies for fine-tuning them.At the end,the article provides insights into future research directions,aiming to reveal more unknown fundamentals of spin-dependent electrocatalysis and encourage further exploration in spin-related research and applications.

spin-dependent electrocatalysisspin configurationspin-related featurescharacterization techniquesmanipulation strategies

Zhengjie Chen、Xiaoning Li、Hao Ma、Yuwei Zhang、Jing Peng、Tianyi Ma、Zhenxiang Cheng、Jose Gracia、Yuanmiao Sun、Zhichuan J.Xu

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Faculty of Materials Science and Energy Engineering,Shenzhen University of Advanced Technology,Shenzhen 518107,China

School of Materials Science and Engineering,Nanyang Technological University,Singapore 639798,Singapore

School of Science,RMIT University,Melbourne 3000,Australia

Institute of Technology for Carbon Neutrality,Shenzhen Institute of Advanced Technology,Chinese Academy of Sciences,Shenzhen 518055,China

Institute for Superconducting and Electronic Materials(ISEM),Faculty of Engineering and Information Sciences,Innovation Campus,University of Wollongong,North Wollongong 2500,Australia

MagnetoCat SL.General Polavieja 931,Alicante 03012,Spain

Center for Advanced Catalysis Science and Technology,Nanyang Technological University,Singapore 639798,Singapore

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National Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaShenzhen Institute of Advanced Technology(SIAT)International Joint Lab ProjectShenzhen Science and Technology ProgramGuangdong Basic and Applied Basic Research FoundationGuangdong Basic and Applied Basic Research FoundationScience and Technology Foundation of ShenzhenSingapore Ministry of Education Tier 1 Grant

5237323352403381E3G113KQTD202211010936470582022A15151104082023B1515020102JCYJ20230807140900001RG78/22

2024

10.1093/nsr/nwae314

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ISSN：
年,卷(期)：2024.11(9)