Recent advances in microenvironment regulation for electrocatalysis

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外文摘要：High-efficiency electrocatalysis could serve as the bridge that connects renewable energy technologies,hydrogen economy and carbon capture/utilization,promising a sustainable future for humankind.It is therefore of paramount significance to explore feasible strategies to modulate the relevant electrocatalytic reactions and optimize device performances so as to promote their large-scale practical applications.Microenvironment regulation at the catalytic interface has been demonstrated to be capable of effectively enhancing the reaction rates and improving the selectivities for specific products.In this review we summarize the latest advances in microenvironment regulation in typical electrocatalytic processes(including water electrolysis,hydrogen-oxygen fuel cells,and carbon dioxide reduction)and the related in situ/operando characterization techniques and theoretical simulation methods.At the end of this article,we present an outlook on development trends and possible future directions.

外文关键词：

microenvironment regulationelectrical double layerhydrogen electrocatalysisoxygen electrocatalysisCO2 reduction reaction

作者：

Zhiyuan Xu、Xin Tan、Chang Chen、Xingdong Wang、Rui Sui、Zhongbin Zhuang、Chao Zhang、Chen Chen

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作者单位：

Engineering Research Center of Advanced Rare Earth Materials,Department of Chemistry,Tsinghua University,Beijing 100084,China

Research Institute of Petroleum Processing,SINOPEC,Beijing 100083,China

State Key Lab of Organic-Inorganic Composites,Beijing University of Chemical Technology,Beijing 100029,China

MOE International Joint Laboratory of Materials Microstructure,Institute for New Energy Materials and Low-Carbon Technologies,School of Materials Science and Engineering,Tianjin University of Technology,Tianjin 300384,China

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出版年：

2024

DOI：

10.1093/nsr/nwae315

国家科学评论(英文版)

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ISSN：

年,卷(期)：2024.11(12)