首页|固废基硫掺杂多孔炭材料制备及其对CO2吸附性能研究进展

固废基硫掺杂多孔炭材料制备及其对CO2吸附性能研究进展

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含碳固废来源广、产量大,其大量堆存严重制约了环境可持续发展,因此含碳固废资源化利用意义重大.利用含碳固废制备多孔炭材料是其清洁高效利用的重要方式之一.对多孔炭进行硫原子掺杂不仅可使材料表面的亲水性得到改善,还可以改变材料表面的化学异质性,生成有利于CO2捕集的活性位点,强化材料对CO2分子的吸附作用,从而提高其CO2吸附容量.简述了固废基硫掺杂多孔炭材料的制备方法,总结了硫掺杂多孔炭材料用于CO2吸附的最新研究进展,并对硫掺杂多孔炭材料未来发展趋势及其在CO2吸附领域的工业化应用进行了展望.
Progress in preparation and CO2 adsorption properties of solid waste-based sulfur-doped porous carbon materials
Carbon-containing solid wastes have a wide range of sources as well as large output,which seriously restricts the sustainable development of the environment.Therefore,the resource utilization of carbon-containing solid waste is of great significance.The preparation of porous carbon from carbon-containing solid wastes is one of the most important ways to utilize them cleanly and efficiently.Sulfur atom doping of porous carbon can not only improve the hydrophilicity of the material surface,but also changes the chemical heterogeneity,and then generates active sites favorable for CO2 capture,strengthens the adsorption performance of CO2 molecules by the material,thus increases the adsorption capacity of CO2.This paper briefly describes the preparation method of solid waste-based sulfur-doped porous carbon materials,summarizes the latest research progress of sulfur-doped porous carbon materials for CO2 adsorption,and looks forward to the future development trend of sulfur-doped porous carbon materials and their industrialized application in the field of CO2 adsorption.

waste treatmentcarbon containing solid wastesulfur-doped porous carbonadsorbentsCO2 capture

王宝凤、王术高、程芳琴

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山西大学资源与环境工程研究所,CO2减排与资源化利用教育部工程研究中心,山西 太原 030006

废物处理 含碳固废 硫掺杂多孔炭 吸附剂 CO2捕集

国家自然科学基金山西省区域合作项目山西省研究生教育创新项目

221782042021040411010292022Y134

2024

化工学报
中国化工学会 化学工业出版社

化工学报

CSTPCD北大核心
影响因子:1.26
ISSN:0438-1157
年,卷(期):2024.75(2)
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