化工学报2024,Vol.75Issue(8) :2991-3001.DOI:10.11949/0438-1157.20240219

中心脉冲气-液-固循环流化床微生物燃料电池产电特性

Power generation characteristics of central pulse gas-liquid-solid circulating fluidized bed microbial fuel cell

朱楼 宋杨凡 王猛 施睿鹏 厉彦民 陈鸿伟 刘卓 魏翔
化工学报2024,Vol.75Issue(8) :2991-3001.DOI:10.11949/0438-1157.20240219

中心脉冲气-液-固循环流化床微生物燃料电池产电特性

Power generation characteristics of central pulse gas-liquid-solid circulating fluidized bed microbial fuel cell

朱楼 1宋杨凡 1王猛 1施睿鹏 1厉彦民 1陈鸿伟 1刘卓 1魏翔1
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作者信息

  • 1. 华北电力大学河北省低碳高效发电技术重点实验室,河北 保定 071000
  • 折叠

摘要

为进一步提升微生物燃料电池(MFC)的电化学性能,设计并搭建了一个中心脉冲气-液-固循环流化床微生物燃料电池(CPCFB-MFC),通过设计多组实验工况研究了脉冲液流频率和幅值、颗粒循环速率及气体流量对CPCFB-MFC产电及污水处理特性的影响.在中心液流脉冲频率为0.25 Hz、脉冲幅值为0.08 m/s、颗粒循环速率为3.3 kg/(m2·s)、气体流量为2 L/min条件下,CPCFB-MFC的输出电压达到最高(为649.2 mV),此时污水处理时间最短(为77 h).通过对比不同工况的污水处理效率和综合能耗,证明了在反应器内采用脉冲液流和气-液-固循环运行方式能进一步提升MFC的综合性能.这项工作对推动微生物燃料电池技术的产业化具有重要意义.

Abstract

In order to further improve the electrochemical performance of microbial fuel cell(MFC),a central pulse gas-liquid-solid circulating fluidized bed microbial fuel cell reactor(CPCFB-MFC)was designed and constructed.The effects of pulse liquid flow frequency,amplitude,particle circulation rate,and gas flow rate on the power generation and sewage treatment characteristics of CPCFB-MFC were studied by designing multiple experimental conditions.Under the conditions of central liquid flow pulse frequency of 0.25 Hz,pulse amplitude of 0.08 m/s,particle circulation rate of 3.3 kg/(m2·s)and gas flow of 2 L/min,the output voltage of CPCFB-MFC reached the highest,which was 649.2 mV,and the sewage treatment time was the shortest,which was 77 h.By comparing the sewage treatment efficiency and comprehensive energy consumption under different operating conditions,it can be proven that the adoption of pulse liquid flow and gas-liquid-solid multiphase operation can further improve the comprehensive performance of MFC reactors.This work is of great significance for promoting the industrialization of microbial fuel cell technology.

关键词

微生物燃料电池/循环流化床/脉冲液流/产电/污水处理/活性炭

Key words

microbial fuel cell/circulating fluidized bed/pulse liquid flow/electricity generation/sewage treatment/activated carbon

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基金项目

国家自然科学基金项目(52106199)

河北省自然科学基金项目(E2023502067)

河北省教育厅科学研究项目(BJK2024065)

中央高校基本科研业务费专项资金(2023MS122)

出版年

2024
化工学报
中国化工学会 化学工业出版社

化工学报

CSTPCDCSCD北大核心
影响因子:1.26
ISSN:0438-1157
参考文献量36
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