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废弃生物质水热炭化衍生碳基光催化材料的研究进展

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水热炭化是一种经济且环境友好的废弃生物质热化学转化技术。废弃生物质通过水热炭化制备碳基光催化材料,不仅可实现废弃物的高值利用,而且可通过光催化材料的的应用缓解环境污染和能源危机。本综述将水热炭化制备的废弃生物质碳基光催化材料分成水热炭、碳点和碳基复合材料三类,并系统总结其制备、光催化机理和应用方面的研究进展。首先,归纳了3种光催化剂的制备,包括形成机理和物化结构;然后分别阐述了各类催化剂的光催化过程和光催化性能提高途径,以及从有机污染物降解、重金属去除、消毒、产氢和CO2还原等领域介绍了光催化应用;最后,对该领域未来的研究重点和发展方向进行了展望。
Research progress on waste-biomass-derived carbon-based photocatalysts by hydrothermal carbonization
Hydrothermal carbonization(HTC)is a facile and environmentally friendly thermochemical conversion technique for waste biomass.The preparation of carbon-based photocatalysts from waste biomass by HTC can realize the value-added utilization of waste and alleviate environmental pollution and energy crisis through photocatalytic applications.In this review,photocatalysts derived from waste-biomass by HTC are divided into three categories:hydrochars,carbon dots,and carbon-based composite photocatalysts,and their research progress in preparation,photocatalytic mechanism,and application is comprehensively summarized.Firstly,the synthesis of these photocatalysts,including the formation mechanism and the physicochemical properties of the products,is outlined.Secondly,the photocatalytic process and performance improvement methods of three types of photocatalysts are described,respectively.Thirdly,the photocatalytic applications in organic pollutant degradation,heavy metal removal,disinfection,hydrogen production,and CO2 reduction are listed.Finally,the future research focus and development direction in this field are prospected.

waste biomasshydrothermal carbonizationhydrocharcarbon dotscarbon-based photocatalystphotocatalysis

缪巍、陈则良、刘振刚、罗磊

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中国城市建设研究院有限公司,北京,100120

中国科学院生态环境研究中心,北京,100085

废弃生物质 水热炭化 水热炭 碳点 碳基光催化剂 光催化

国家自然科学基金

21876188

2024

环境化学
中国科学院生态环境研究中心

环境化学

CSTPCD北大核心
影响因子:1.049
ISSN:0254-6108
年,卷(期):2024.43(1)
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