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朔州东部农田土壤-农作物重金属富集及健康风险评价

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为研究重金属在农田土壤-作物之间的累积性及人群健康风险,采用富集因子(EF)、地累积指数(Igeo)和潜在生态危害指数(RI)等指标对山西省朔州市东部三县市(山阴县、应县、怀仁市)131个样点农田土壤-作物系统(玉米、高粱和大豆)中重金属的含量、来源及富集程度进行调查,并采用EPA推荐的风险评估模型对人群健康风险进行了评估。结果表明:1)研究区土壤中8种重金属(Cd、Cr、As、Hg、Pb、Cu、Zn、Ni)含量均未超过《土壤环境质量农用地土壤污染风险管控标准(试行)》(GB 15618-2018)中农用地土壤污染风险筛选值;而Cr、Hg、Pb的平均含量分别是研究区背景值的1。20倍、6。26倍和1。33倍。2)研究区土壤中Hg元素为显著富集,其余重金属无富集。地累积指数分级结果表明,土壤中Hg呈中度污染,其余为无污染。潜在生态危害指数结果表明研究区为中度污染水平。3)主成分分析结果表明,研究区Ni、Cr、Zn、Cu主要来源于"自然来源",Hg主要来源于"直接工业源",As、Pb主要来源于"大气沉降-工业源",而Cd主要来自"农业来源"。4)8种重金属对儿童的非致癌风险高于成人。研究区Pb对儿童和成人均无致癌风险,Cd和As对儿童和成人的致癌风险均处于可接受范围内,而Cr、Ni是主要致癌风险因子。
Evaluation of heavy metal enrichment and health risks in agricultural soils-crops in eastern Shuozhou,Shanxi Province,China
In order to study the accumulation of heavy metals between farmland soil and crops and the health risks of pollution,the content of 8 different heavy metals included Cd,Cr,As,Hg,Pb,Cu,Zn,and Ni in the soil and crop(corn,sorghum,and soybean)collected from 131 sites in three different country and city in eastern Shuozhou,Shanxi Province,China were determined,and various indices such as enrichment factors(EF),geo-accumulation index(Igeo)and potential ecological hazard index(RI)were used to survey the polluted degree of soil-crop systems and the pollution source.Also,the health risk was assessed based on the risk model recommended by EPA.The results showed that:1)The concentrations of eight heavy metals(Cd,Cr,As,Hg,Pb,Cu,Zn,Ni)in the soil of the study area did not exceed the limit values stipulated in the"Soil Environmental Quality Risk Control Standard for Soil Contamination of Agricultural Land(Trial)"(GB15618-2018);while the average levels of Cr,Hg,and Pb were 1.20,6.26 and 1.33 times higher than the background values in the study area,respectively.2)Hg in the soil of the study area was significantly enriched,while the rest of the heavy metals were not enriched.The results of the ground accumulation index classification show that Hg was moderately contaminated and the rest was non-contaminated.The results of the Potential Ecological Hazard Index indicated the study area was moderately polluted.3)The results of the principal component analysis show that Ni,Cr,Zn,and Cu in the study area mainly come from"natural sources",Hg mainly comes from"direct industrial sources",As and Pb mainly come from"atmospheric deposition-industrial sources",and Cd Mainly from"agricultural sources".4)The non-carcinogenic risks of 8 heavy metals in children are higher than those in adults.In the study area,Pb had no carcinogenic risk to children and adults,and the carcinogenic risks of Cd and As to children and adults were within an acceptable range,while Cr and Ni were the main carcinogenic risk factors.

farmland soilcropsheavy metalsenrichment factorhealth risk assessment

张娟、王明君、郭掌珍

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山西中环宏达环境检测技术有限公司,太原,030032

山西农业大学资源环境学院,太谷,030801

山西农业大学环境监测有限公司,太谷,030801

农田土壤 农作物 重金属 富集因子 健康风险评价

土壤环境与养分资源山西省重点实验开放基金

2017003

2024

环境化学
中国科学院生态环境研究中心

环境化学

CSTPCD北大核心
影响因子:1.049
ISSN:0254-6108
年,卷(期):2024.43(4)
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