环境化学2024,Vol.43Issue(12) :4082-4092.DOI:10.7524/j.issn.0254-6108.2023061302

长江中下游典型湖泊鱼体中多环芳烃(PAHs)的污染特征及风险评价

Pollution characteristics and risk assessment of polycyclic aromatic hydrocarbons(PAHs)in fish of typical lakes in the middle and lower reaches of the Yangtze River

秦海娇 史秋月 王永强 毕斌 张森霖 刘宪斌 李琳琳 杨莉园 卢少勇
环境化学2024,Vol.43Issue(12) :4082-4092.DOI:10.7524/j.issn.0254-6108.2023061302

长江中下游典型湖泊鱼体中多环芳烃(PAHs)的污染特征及风险评价

Pollution characteristics and risk assessment of polycyclic aromatic hydrocarbons(PAHs)in fish of typical lakes in the middle and lower reaches of the Yangtze River

秦海娇 1史秋月 2王永强 2毕斌 2张森霖 2刘宪斌 3李琳琳 2杨莉园 2卢少勇2
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作者信息

  • 1. 中国环境科学研究院国家环境保护湖泊污染控制重点实验室,湖泊水污染治理与生态修复国家工程实验室,北京,100012;天津科技大学海洋与环境学院,天津,300457
  • 2. 中国环境科学研究院国家环境保护湖泊污染控制重点实验室,湖泊水污染治理与生态修复国家工程实验室,北京,100012
  • 3. 天津科技大学海洋与环境学院,天津,300457
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摘要

为揭示长江中下游4个典型湖泊(鄱阳湖、洞庭湖、东江湖和梁子湖)鱼体中多环芳烃(PAHs)的污染特征和风险水平,检测了 20种鱼样中的16种PAHs,分析了 PAHs污染水平,并开展了风险评价.结果表明16种PAHs共检出11种,∑PAHs的含量分别为鄱阳湖(32.59-39.81 ng·g-1)、洞庭湖(29.47-37.60 ng·g-1)、东江湖(26.07-36.25 ng·g-1)和梁子湖(27.78-47.95 ng·g-1).主要检出物质有5种分别是苯并[b]荧蒽、苯并[k]荧蒽、芘、䓛和芴,其中苯并[b]荧蒽的检出率和检出浓度最高.苊烯、苊、茚并[1,2,3-cd]芘、二苯并[a,h]蒽和苯并[g,h,i]芘在所有鱼体内均未检出.4个湖泊鱼体内PAHs污染水平与国内外相比较低.健康风险评价结果显示,4个湖泊的非致癌风险指数(HI)均小于1,不会对人体产生非致癌风险;但致癌风险值(R)均超过了 10-6,表明可能会对人体产生致癌风险,应引起重视.

Abstract

In order to reveal the pollution characteristics and risk levels of polycyclic aromatic hydrocarbons(PAHs)in fish from four typical lakes(Poyang Lake,Dongting Lake,Dongjiang Lake and Liangzi Lake)in the middle and lower reaches of the Yangtze River,16 PAHs in 20 fishes were detected,the levels of PAHs contamination were analyzed,and the risk assessment was carried out.The results showed that 11 PAHs were detected,with the concentrations of 32.59-39.81 ng·g-1 in Poyang Lake,29.47-37.60 ng·g-1 in Dongting Lake,26.07-36.25 ng·g-1 in Dongjiang Lake and 27.78-47.95 ng g-1 in Liangzi Lake.The main detected substances were benzo[b]fluoranthene,benzo[k]fluoranthene,pyrene,chrysene and fluorene,of which benzo[b]fluoranthene had the highest detection rate and concentration.Acenaphthylene,acenaphthene,indeno[1,2,3-cd]pyrene,dibenzo[a,h]anthracene and benzo[g,h,i]perylene were not detected in all fish.The levels of PAHs pollution in fish in four lakes were relatively low compared to those at home and abroad.The health risk assessment results showed that the non-carcinogenic risk index of four lakes were all less than 1,which would not cause non-carcinogenic risks to human body.The carcinogenic risk index were all over 10-6,indicating that it might be carcinogenic risk to human body,to which more attention should be paid.

关键词

长江中下游典型湖泊/鱼体/多环芳烃(PAHs)/污染特征/风险评价

Key words

The middle and lower reaches of the Yangtze River/fish/polycyclic aromatic hydrocarbons(PAHs)/pollution levels/health risk

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出版年

2024
环境化学
中国科学院生态环境研究中心

环境化学

CSTPCDCSCD北大核心
影响因子:1.049
ISSN:0254-6108
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