首页|农田土壤和辣椒/甘薯可食部位镉砷铅污染特征及健康风险评价

农田土壤和辣椒/甘薯可食部位镉砷铅污染特征及健康风险评价

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为探明农田土壤重金属Cd、As和Pb及其在作物可食部位的含量特征,在金属冶炼和污水灌溉共同影响的农田区域,重点调查分析了土壤、辣椒与甘薯可食部位(两种作物果实分别在地上和地下)中Cd、As和Pb含量及污染特征,并采用化学致癌物模型和化学非致癌物模型对两种作物果实及不同部位进行了人体健康风险评价。结果表明,辣椒和甘薯农田土壤Cd和As达中度复合污染水平,且距离污染源较近的甘薯农田土壤Cd、As和Pb综合污染指数(2。82)显著高于辣椒农田(2。38)(P<0。05)。然而,甘薯可食部位Cd、As和Pb含量均未超过《食品安全国家标准食品中污染物限量》(GB 2762-2022),全部辣椒果实Cd含量超过《绿色食品辣椒制品》国家农业行业标准(NY/T 1711-2020)。进一步分析发现辣椒可食部位对土壤中Cd、As和Pb的富集系数显著高于甘薯,尤其是对土壤Cd具有很强的富集能力,可见富集系数是决定辣椒果实Cd累积的主要因子。对辣椒和甘薯可食部位中化学致癌物Cd和As的健康风险进行评价表明,辣椒果实中Cd累积对成人有较显著健康风险(Ri>1×10-4),辣椒和甘薯可食部位均对儿童有可接受的健康风险,二者中非致癌物Pb尚未对人体产生健康风险。总之,Cd和As中度复合污染区生产的辣椒果实对Cd的富集能力很强,已构成显著的人体健康风险,甘薯则存在可接受水平的健康风险。
Characteristics of Cd,As,and Pb Pollution in Farmland Soil and Edible Parts of Chili Pepper and Sweet Potato and Their Health Risk Assessment
To clarify the characteristics of Cd,As,and Pb concentrations in edible parts of crops and farmland soils,a key farmland survey was conducted on the field scale to investigate the characteristics of Cd,As,and Pb in soil and chili pepper(edible parts in the above-ground section)and sweet potato(edible parts under the ground)and assess the health risk of Cd-As-Pb in edible parts of chili pepper and sweet potato to humans in the typical co-contaminated agricultural soils by Cd,As,and Pb from metal smelting and sewage irrigation in North China.The results showed that the agricultural soil from chili pepper and sweet potato fields was co-contaminated by Cd and As at a moderate pollution level.The combined pollution index(2.82)of soil from sweet potato farmland was significantly higher than that from chili pepper fields(2.38)for sweet potato land much nearer to the pollution sources(P<0.05).However,Cd concentrations in edible parts of chili pepper exceeded the safety limitation of 0.1 mg·kg-1 in the national standard of"Green food pepper products"(NY/T 1711-2020),but the concentrations of Cd,As,and Pb in edible parts of sweet potato did not exceed the"National food safety standard food pollutant limit"(GB 2762-2022).Additionally,the bioaccumulation factors(BAFs)of Cd,As,and Pb in edible parts of chili pepper to soil were markedly higher than those of sweet potatoes,especially for Cd,which showed the maximum of the BAFs for chili pepper.Therefore,BAFs could be the key factor in Cd accumulation in the fruits of chili peppers.The risk assessment of Cd and As as the carcinogenic elements in edible parts of chili pepper and sweet potato to human health demonstrated that Cd in the whole fruit of chili pepper had posed a significant health risk to adults(Ri>1 × 10-4),and it was an acceptable level of health risk from Cd and As in edible parts of both crops to children.The non-carcinogenic element of Pb in the fruits of both crops did not cause health risks to adults or children.In summary,the chili pepper products from this co-contaminated farmland by Cd and As would pose risks to human health,and the sweet potato products would cause acceptable health risks to humans.

co-contaminated farmland by heavy metalschilipeppersweetpotatocadmium(Cd)-arsenic(As)-lead(Pb)contamination characteristicshealth risk

张志强、韦亮、耿丽平、刘峰、赵全利、吴鸿斌、薛培英、刘文菊

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河北农业大学资源与环境科学学院,省部共建华北作物改良与调控国家重点实验室,河北省农田生态环境重点实验室,保定 071000

河北省农业环境保护监测总站,石家庄 050035

重金属复合土壤 辣椒 甘薯 镉(Cd)-砷(As)-铅(Pb) 污染特征 健康风险

2025

环境科学
中国科学院生态环境研究中心

环境科学

北大核心
影响因子:1.913
ISSN:0250-3301
年,卷(期):2025.46(1)