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淮河中下游地区大气CH4浓度及变化特征研究

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基于2023年安徽省五河高精度温室气体浓度观测站大气CH4浓度数据及同期气象观测数据,研究了淮河中下游地区典型下垫面状态下CH4浓度变化特征、输送影响及潜在排放源区分布特征。结果表明:具有区域代表性的CH4浓度为(2113。0±1。9)×10-9,远低于受到观测站附近局地影响的CH4浓度((2417。4±9。9)×10-9);五河地区CH4浓度日变化在不同季节均呈现出早上高、午后低的峰谷特征,月变化呈现夏高冬低的单峰特征,低层(50 m)和高层(80 m)CH4浓度差异日间小、夜晚大。地面风对五河地区CH4浓度影响显著,易受到西南扇区气流的影响而升高;CH4浓度随着风速的增加而下降。后向轨迹和潜在源解析表明,排放区域主要分布在中部四省(安徽、河南、湖北、江西)、江苏省和山东省,这些区域内分布着大量的湿地、水稻田及畜牧业生产基地,均是淮河中下游典型代表性地区CH4浓度升高的主要影响因素。
The variation characteristics of atmospheric CH4 mixing ratio observed in the middle and lower reaches of the Huai River
Based on the atmospheric CH4 mixing ratios from the high-precision greenhouse gas monitoring station in Wuhe,Anhui Province in 2023,as well as the concurrent meteorological observation data,this study investigated the CH4 mixing ratio variation characteristics,transport influence,and potential emission source distribution characteristics in the typical underlying surface conditions of the middle and lower reaches of the Huai River.The results show that the CH4 mixing ratios with regional representativeness is(2113.0±1.9)×10-9,which is significantly lower than the CH4 mixing ratio affected by local conditions near the monitoring station((2417.4±9.9)×10-9).The CH4 mixing ratios in the Wuhe area exhibits a peak-trough feature with higher levels in the morning and lower levels in the afternoon in different seasons,and a unimodal feature with higher levels in summer and lower levels in winter.The difference in CH4 mixing ratios between the lower layer(50 m)and the upper layer(80 m)is small during the day and large at night.The ground wind has asignificant impact on the CH4 mixing ratios in the Wuhe area,which is easily influenced by the southwest sector airflow and increases;the CH4 mixing ratios decrease with the increase of wind speed.Backward trajectory and potential source analysis indicate that the emission areas are mainly distributed in the four provinces of Central China(Anhui,Henan,Hubei,Jiangxi),Jiangsu Province,and Shandong Province,where there are a large number of wetlands,paddy fields,and livestock production bases,all of which are the main factors affecting the increase of CH4 mixing ratios in the typical representative areas of the middle and lower reaches of the Huai River.

the middle and lower reaches of the Huai RiverCH4variation of mixing ratiospotential emission sources

王蒙、沈玉亮、杨关盈、张元刚、田晓明、孙荣华、张浩、霍彦峰、汪义兰

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安徽省气象信息中心,合肥 230031

安徽省气象科学研究所,大气科学与卫星遥感安徽省重点实验室,合肥 230031

寿县国家气候观象台,中国气象局淮河流域典型农田生态气象野外科学试验基地,寿县 232200

安徽省大气探测技术保障中心,合肥 230031

蚌埠市五河县气象局,蚌埠 233300

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淮河中下游 CH4 浓度变化特征 潜在排放源

2025

环境科学学报
中国科学院生态环境研究中心

环境科学学报

北大核心
影响因子:1.645
ISSN:0253-2468
年,卷(期):2025.45(1)