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早期遗址化石ESR测年等效剂量拟合函数的选择

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在动物牙齿化石样品电子自旋共振测年(Electron Spin Resonance Dating,ESR)中辐照剂量点拟合函数的选择对等效剂量DE的确定至关重要.目前,早期遗址老化石(>1 Ma)的DE拟合常采用双饱和指数(Double Saturation Exponential,DSE)函数,使用该函数时一般需要15个以上剂量点和大于20 kGy的最大辐照剂量(Dmax)才能保证DE值的拟合精度.但在实际应用中存在部分老化石的样品量较少,且缺乏大剂量辐照的准确标定情况,导致无法满足上述DSE函数的适用条件.本研究对涵盖晚中新世至早更新世的化石样品进行了不同拟合函数的对比分析,着重探讨单饱和指数(Single Saturation Exponential,SSE)函数在老化石样品DE拟合中的适用性.研究表明:对11~15个剂量点进行拟合时,对于2 000 Gy<DE<4 500 Gy和DE>4 500 Gy的样品,分别在1.9×DE<Dmax<3.5×DE和Dmax≥6.5×DE条件下采用SSE函数拟合,可以获得与使用DSE函数基本一致的DE结果.
The choice of equivalent dose fitting function in ESR dating of old fossil samples
[Background]In electron spin resonance dating(ESR)of old fossils,the double saturation exponential(DSE)function is often used for the equivalent dose(DE)determination,it generally requires more than 15 dose points and the maximum irradiation dose(Dmax)greater than 20 kGy to ensure the fitting accuracy,which limit the practical application of dating old fossils by ESR method with insufficient sample size.[Purpose]This study aims to explore the feasibility and reliability of using the single saturation exponential(SSE)fitting function to fit fewer dose points with lower Dmax to obtain the DE values of the fossil teeth from the late Miocene to the early Pleistocene,and compared with the ones determined by DSE function.[Methods]Firstly,17 fossil samples were taken from seven fossil sites in different regions of China and Myanmar,and their ages covered the late Miocene to early Pleistocene.Then,three fitting functions,i.e.,DSE,SSE and EPL-exponential plus linear,were employed to obtain the DE values of ESR using the additional dose method.Finally,the influence of different Dmax on the DE results of three fitting functions was investigated by comparative analysis.[Results]Comparison results show that:(1)The SSE and DSE function are used to fit the 15 dose points with Dmax=50 kGy,and the DE-SSE results of 11 samples are basically consistent with the DE-DSE results,meanwhile the precision of the fitting results of SSE function is generally higher than DSE cases.(2)For samples with DE>4 500 Gy and 2 000 Gy<DE<4 500 Gy,the results of SSE and DSE are basically consistent within the error range under the conditions of Dmax≥6.5×DE and 1.9×DE<Dmax<3.5×DE,respectively,which can provide the recommended dose value of Dmax for samples with DE>2 000 Gy when using SSE function.(3)For fossil samples with 2 000 Gy<DE<4 500 Gy,the SSE function can be used to fit the 11 dose points with Dmax≤10 kGy,and the DE results are generally consistent with the DSE function within the error range.[Conclusions]Based on above results,it is viable to use SSE function to perform DE fitting on old fossil samples under certain Dmax/DE conditions,and establishing the standardized growth curve of old fossils and the fragmental analysis of the fossil teeth for DE determination will be explored in the future study.

Fossil teethESR datingEquivalent doseFitting function

谢君绮、韩非、柳华霖、黄曼琛、高峰

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云南大学 地球系统科学重点实验室 昆明 650500

云南省文物考古研究所 昆明 650118

牙化石 ESR测年 等效剂量 拟合函数

2025

核技术
中国核学会 中国科学院上海应用物理研究所

核技术

北大核心
影响因子:0.299
ISSN:0253-3219
年,卷(期):2025.48(1)