首页|基于CFD-PBE耦合的连续结晶过程数值模拟

基于CFD-PBE耦合的连续结晶过程数值模拟

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通过CFD(计算流体力学)与PBE(粒数衡算方程)耦合对连续结晶过程进行数值模拟.采用QMOM(积分矩方法)求解PBE.在考虑成核、生长、聚并和破碎的情况下,通过网格独立性验证确定计算网格数量.在此基础上研究挡板设置、停留时间、搅拌转速以及搅拌桨类型等因素对CSD(晶体粒径分布)演变的影响,结果表明:挡板的设置增强了结晶器内湍流程度;高转速和低停留时间会获得平均粒径较小的颗粒.对比3种搅拌桨对CSD演变的影响,轴流式的螺旋桨功耗小,适用于大颗粒晶体结晶过程,而径流式的圆盘涡轮桨适用于微粒结晶过程.
Numerical simulation of continuous crystallization process based on CFD-PBE coupling model
The continuous crystallization process was numerically simulated by coupling CFD-PBM(computational fluid dynamics and population balance model).QMOM was employed to solve the coupled PBE.When nucleation,growth,coalescence and breakage were considered,the number of grids for numerical simulation were determined by the grid independence verification.Then the effect of baffle installment,residence time,rotating speed and impeller type on the CSD evolution was investigated.The results show that the turbulence intensity is improved by setting up the baffle in the crystallizer.Smaller particle size is obtained with high rotational speed and low residence time.Finally,comparing the CSD from three impellers,the axial flow propeller shows to be lower power consumption and suitable for crystallization with large particle size,while radial disc turbine propeller can be selected to obtain microparticle crystal.

continuous crystallizationnumerical simulationpopulation balance equationquadrature method of momentcrystal size distribution

潘立杰、刘伯潭、赵文立、盖晓龙

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天津科技大学化学工程与材料科学学院,天津 300457

天津大学化学工程联合国家重点实验室,天津 300350

连续结晶 数值模拟 粒数衡算方程 积分矩方法 晶体粒径分布

国家自然科学基金资助项目

21978218

2024

化学工程
华陆工程科技有限责任公司

化学工程

CSTPCD北大核心
影响因子:0.438
ISSN:1005-9954
年,卷(期):2024.52(1)
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