二维层状沸石的合成及其催化、吸附与分离应用
Synthesis of Two-Dimensional Layered Zeolites and Their Catalysis,Adsorption and Separation Applications
胡诗雨 1闫玥儿 2张亚红 1王振东 3唐颐1
作者信息
- 1. 复旦大学 化学系 上海 200438
- 2. 复旦大学 中华古籍保护研究院 上海 200433
- 3. 中石化(上海)石油化工研究院有限公司 绿色化工与工业催化全国重点实验室 上海 201208
- 折叠
摘要
与三维沸石相比,二维层状沸石具有更大的表面积、更短的扩散距离和更具韧性的结构,在许多领域中都具有更大优势.近年来,二维层状沸石的研究已成为新热点.本文基于前期文献调研总结,从两类合成角度(Bottom-up和Top-down法)归纳了近年来二维沸石的合成方法,重点综述了同种类型沸石的不同合成法的进展.此外,本文简述了二维沸石在催化、吸附和分离领域中的应用,并展望了二维沸石广阔的应用前景,以期为二维沸石的合成与应用提供参考.
Abstract
Compared with three-dimensional zeolites,two-dimensional layered zeolites have greater advantages in many fields,with larger surface area,shorter diffusion distance and more ductile structure.In recent years,the research on two-dimensional layered zeolites has become a new hotspot.Based on previous research and summary,this article summarizes the synthesis methods of two-dimensional zeolites in the past five years from two types of synthesis perspectives(bottom-up and top-down methods),with a focus on reviewing the progress of different synthesis methods for the same topology of zeolite.In addition,this article briefly describes the applications of two-dimensional zeolites in the fields of catalysis,adsorption,and separation and looks forward to the broad application prospects of two-dimensional zeolites so as to provide theoretical guidance and reference basis for the synthesis and application of two-dimensional zeolites.
关键词
二维沸石/合成/酸催化/吸附/分离膜Key words
2D zeolite/synthesis/acid catalysis/adsorption/separation membrane引用本文复制引用
基金项目
国家重点研发计划(2018YFA0209402)
国家自然科学基金(22072028)
国家自然科学基金(22088101)
上海市自然科学基金(22ZR1407200)
出版年
2024
NETL
NSTL
万方数据