净水技术2024,Vol.43Issue(3) :16-28.DOI:10.15890/j.cnki.jsjs.2024.03.003

污水深度处理中常见固相臭氧催化剂及其催化机理综述

Overview of Common Solid-Phase Ozone Catalysts and Catalytic Mechanism in Waste water Advanced Treatment

李旭芳 沈鹏飞 马鲁铭
净水技术2024,Vol.43Issue(3) :16-28.DOI:10.15890/j.cnki.jsjs.2024.03.003

污水深度处理中常见固相臭氧催化剂及其催化机理综述

Overview of Common Solid-Phase Ozone Catalysts and Catalytic Mechanism in Waste water Advanced Treatment

李旭芳 1沈鹏飞 1马鲁铭2
扫码查看

作者信息

  • 1. 中国铁工投资建设集团有限公司,北京 101300;中国中铁生态环境专业研发中心,上海 200331
  • 2. 同济大学环境科学与工程学院,上海 200092
  • 折叠

摘要

近年来,催化臭氧氧化工艺由于对有机物去除率高、污水处理效果好,在污水深度处理中的研究和应用逐渐广泛和深入.催化臭氧氧化工艺的核心在于,在催化剂的作用下,羟基自由基(·OH)浓度显著提升,从而强化污水处理效果.因此,催化剂的开发是催化臭氧氧化工艺应用研究的关键.文章总结了不含载体的、可直接作为有效成分的催化剂,如铁(Fe)、锰(Mn)、铈(Ce)、镍(Ni)、钴(Co)、钛(Ti)等金属及其氧化物,以及活性炭、碳纳米管、石墨烯等碳材料催化臭氧的效果和可能的催化机理,分析了当前研究较多的催化剂在实际应用中可能存在的问题,为催化剂的研究、开发和应用提供理论基础.

Abstract

In recent years,research and application of catalytic ozonation process is more extensive and in-depth in wastewater advanced treatment,because of high organic pollutants removal rate and good wastewater treatment effect.The core of the catalytic ozonation process is that under the action of the catalyst,the concentration of hydroxyl free radicals(·OH)is significantly increased,thus enhancing the effect of sewage treatment.One key point of catalytic ozonation process is catalyst development.In this paper,several solid-phase catalysts without support material and their catalytic effect and mechanisms are summarized,including metal and metal oxides(eg:iron,manganese,cerium,nickel,cobalt,and titanium)and carbon materials(eg:active carbon,carbon nano tube,and graphene).In addition,the possible problems in practical application of these catalysts are also analyzed.The review can provide a theoretical basis for the continuous development and application of catalysts in catalytic ozonation process.

关键词

催化机理/金属及其氧化物/碳材料/催化臭氧氧化/污水深度处理

Key words

catalytic mechanism/metal and metal oxide/carbon material/catalytic ozonation/wastewater advanced treatment

引用本文复制引用

基金项目

国家自然科学基金(21876111)

出版年

2024
净水技术
上海市净水技术学会,上海市城乡建设和交通委员会科学技术委员会办公室

净水技术

CSTPCD
影响因子:0.643
ISSN:1009-0177
参考文献量66
段落导航相关论文