科学通报(英文版)2024，Vol.69Issue(3) ：382-418.DOI:10.1016/j.scib.2023.12.014

Large-n quasi-phase-pure two-dimensional halide perovskite:A toolbox from materials to devices

Zijia Li Yuexin Lin Hao Gu Nan Zhang Bin Wang Hairui Cai Jinfeng Liao Dejian Yu Yiwang Chen Guojia Fang Chao Liang Shengchun Yang Guichuan Xing
科学通报(英文版)2024，Vol.69Issue(3) ：382-418.DOI:10.1016/j.scib.2023.12.014
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Large-n quasi-phase-pure two-dimensional halide perovskite:A toolbox from materials to devices

Zijia Li 1Yuexin Lin 1Hao Gu 2Nan Zhang 1Bin Wang 1Hairui Cai 1Jinfeng Liao 2Dejian Yu 2Yiwang Chen 3Guojia Fang 4Chao Liang 1Shengchun Yang 1Guichuan Xing2
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作者信息

  • 1. MOE Key Laboratory for Nonequilibrium Synthesis and Modulation of Condensed Matter,School of Physics,National Innovation Platform(Center)for Industry-Education Integration of Energy Storage Technology,Xi'an Jiaotong University,Xi'an 710049,China
  • 2. Joint Key Laboratory of the Ministry of Education,Institute of Applied Physics and Materials Engineering,University of Macau,Macao 999078,China
  • 3. National Engineering Research Center for Carbohydrate Synthesis,Key Laboratory of Fluorine and Silicon for Energy Materials and Chemistry of Ministry of Education,Jiangxi Normal University,Nanchang 330022,China
  • 4. Key Laboratory of Artificial Micro/Nano Structures of Ministry of Education,School of Physics and Technology,Wuhan University,Wuhan 430072,China
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Abstract

Despite their excellent environmental stability,low defect density,and high carrier mobility,large-n quasi-two-dimensional halide perovskites(quasi-2DHPs)feature a limited application scope because of the formation of self-assembled multiple quantum wells(QWs)due to the similar thermal stabilities of large-n phases.However,large-n quasi-phase-pure 2DHPs(quasi-PP-2DHPs)can solve this problem perfectly.This review discusses the structures,formation mechanisms,and photoelectronic and physical properties of quasi-PP-2DHPs,summarises the corresponding single crystals,thin films,and heterojunc-tion preparation methods,and presents the related advances.Moreover,we focus on applications of large-n quasi-PP-2DHPs in solar cells,photodetectors,lasers,light-emitting diodes,and field-effect tran-sistors,discuss the challenges and prospects of these emerging photoelectronic materials,and review the potential technological developments in this area.

Key words

Tow-dimensional halide perovskite/Pure phase/Large-n value/Single crystal/Thin film/Heterojunction

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基金项目

National Natural Science Foundation of China(62105292)

National Natural Science Foundation of China(61935017)

National Natural Science Foundation of China(62175268)

Shaanxi Fundamental Science Research Project for Mathematics and Physics(22JSY015)

Young Talent Fund of Xi'an Association for Science and Technology(959202313020)

Natural Science Foundation of Shaanxi Province(2021GXLH-Z-0)

Natural Science Foundation of Shaanxi Province(2020JZ-02)

Project of Innovative Team of Shaanxi Province(2020TD-001)

China Fundamental Research Funds for the Central Universities,the Science and Technology Development Fund,Macao SAR(FDCT-0044/2020/A1)

China Fundamental Research Funds for the Central Universities,the Science and Technology Development Fund,Macao SAR(006/2022/ALC)

UM's research fund(MYRG2022-00241-IAPME)

UM's research fund(MYRG-CRG2022-00009-FHS)

research fund from Wuyi University(EF38/IAPME-XGC/2022/WYU)

Shenzhen-Hong Kong-Macao Science and Technology Innovation Project(Category C)(SGDX2020110309360100)

出版年

2024
科学通报(英文版)
中国科学院

科学通报(英文版)

CSTPCD
ISSN：1001-6538
参考文献量223
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