Abstract
The water-energy nexus has garnered worldwide interest.Current dual-functional research aimed at co-producing freshwater and electricity faces significant challenges,including sub-optimal capacities("1+1<2"),poor inter-functional coordination,high carbon footprints,and large costs.Mainstream water-to-electricity conversions are often compromised owing to functionality separation and erratic gradients.Herein,we present a sustainable strategy based on renewable biomass that addresses these issues by jointly achieving competitive solar-evaporative desalination and robust clean electricity generation.Using hydrothermally activated basswood,our solar desalination exceeded the 100%efficiency bottle-neck even under reduced solar illumination.Through simple size-tuning,we achieved a high evaporation rate of 3.56 kg h-1 m-2 and an efficiency of 149.1%,representing 128%-251%of recent values without sophisticated surface engineering.By incorporating an electron-ion nexus with interfacial Faradaic elec-tron circulation and co-ion-predominated micro-tunnel hydrodynamic flow,we leveraged free energy from evaporation to generate long-term electricity(0.38 W m-3 for over 14 d),approximately 322%of peer performance levels.This inter-functional nexus strengthened dual functionalities and validated gen-eral engineering practices.Our presented strategy holds significant promise for global human-society-environment sustainability.
基金项目
National Natural Science Foundation of China(U21A20162)
National Natural Science Foundation of China(52261145701)
2115 Talent Development Program of China Agricultural University()