Recent advances in hybrid water electrolysis for energy-saving hydrogen production

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外文摘要：Electricity-driven water splitting to convert water into hydrogen(H2)has been widely regarded as an efficient approach for H2 production.Nevertheless,the energy conversion efficiency of it is greatly limited due to the disadvantage of the sluggish kinetic of oxidation evolution reaction(OER).To effectively address the issue,a novel concept of hybrid water electrolysis has been developed for energy-saving H2 production.This strategy aims to replace the sluggish kinetics of OER by utilizing thermodynamically favorable organics oxidation reaction to replace OER.Herein,recent advances in such water splitting system for boosting H2 evolution under low cell voltage are systematically summarized.Some notable progress of different organics oxidation reactions coupled with hydrogen evolution reaction(HER)are discussed in detail.To facilitate the development of hybrid water electrolysis,the major challenges and perspectives are also proposed.

外文关键词：

Hydrogen evolution reactionHybrid water electrolysisElectrocatalytic oxidationOrganic electro-oxidationHigh-value products

作者：

Di Li、Jibing Tu、Yingying Lu、Bing Zhang

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作者单位：

State Key Laboratory of Chemical Engineering,Institute of Pharmaceutical Engineering,College of Chemical and Biological Engineering,Zhejiang University,Hangzhou,310027,China

ZJU-Hangzhou Global Scientific and Technological Innovation Center,Hangzhou,311215,China

基金：

National Key R&D Program of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaLeading Innovative and Entrepreneur Team Introduction Program of ZhejiangNational Postdoctoral Program for Innovative TalentsChongqing Key Laboratory for Advanced Materials and Technologies of Clean Energies

项目编号：

2018YFA020960022022813218782682019R01006BX20180203JJNY202003

出版年：

2023

绿色化学工程(英文)

中国科学院过程工程研究所

绿色化学工程(英文)

CSCD

ISSN：

年,卷(期)：2023.4(1)

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