首页|Low-energy-consumption temperature swing system for CO2 capture by combining passive radiative cooling and solar heating

Low-energy-consumption temperature swing system for CO2 capture by combining passive radiative cooling and solar heating

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Temperature-swing adsorption(TSA)is an effective technique for CO2 capture,but the temperature swing procedure is energy-intensive.Herein,we report a low-energy-consumption system by combining passive radiative cooling and solar heating for the uptake of CO2 on commercial activated carbons(CACs).During adsorption,the adsorbents are coated with a layer of hierarchically porous poly(vinylidene fluoride-co-hexafluoropropene)[P(VdF-HFP)HP],which cools the adsorbents to a low temperature under sunlight through radiative cooling.For desorption,CACs with broad absorption of the solar spectrum are exposed to light irradiation for heating.The heating and cooling processes are completely driven by solar energy.Adsorption tests under mimicked sunlight using the CACs show that the performance of this system is comparable to that of the traditional ones.Furthermore,under real sunlight irradiation,the adsorption capacity of the CACs can be well maintained after multiple cycles.The present work may inspire the development of new temperature swing procedures with little energy consumption.

CO2 captureSolar heatingPassive radiative coolingTemperature swing adsorption

Ying-Xi Dang、Peng Tan、Bin Hu、Chen Gu、Xiao-Qin Liu、Lin-Bing Sun

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State Key Laboratory of Materials-Oriented Chemical Engineering,Jiangsu National Synergetic Innovation Center for Advanced Materials(SICAM),College of Chemical Engineering,Nanjing Tech University,Nanjing,211816,China

国家杰出青年科学基金国家自然科学基金国家自然科学基金国家自然科学基金

22125804218081102207815521878149

2024

绿色能源与环境(英文)

绿色能源与环境(英文)

CSTPCD
ISSN:
年,卷(期):2024.9(3)
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