Cell-free biocatalysis coupled with photo-catalysis and electro-catalysis:Efficient CC2-to-chemical conversion

扫码查看

原文链接

NETL
NSTL
万方数据

外文摘要：The increasing atmospheric carbon dioxide(CO2)concentration has exposed a series of crises in the earth's ecological environment.How to effectively fix and convert carbon dioxide into products with added value has attracted the attention of many researchers.Cell-free enzyme catalytic system coupled with electrical and light have been a promising attempt in the field of biological carbon fixation in recent years.In this review,the research progresses of photoenzyme catalysis,electroenzyme catalysis and photo-electroenzyme catalysis for converting carbon dioxide into chemical products in cell-free systems are systematically summarized.We focus on reviewing and comparing various coupling methods and principles of photoenzyme catalysis and electroenzyme catalysis in cell-free systems,especially the materials used in the con-struction of the coupling system,and analyze and point out the characteristics and possible problems of different coupling methods.Finally,we discuss the major challenges and prospects of coupling physical signals and cell-free enzymatic catalytic systems in the field of CO2 fixation,suggesting possible strategies to improve the carbon sequestration capacity of such systems.

外文关键词：

CO2 fixationCell-free systemEnzymePhotoenzyme catalysisElectroenzyme catalysis

作者：

Junzhu Yang、Chi-Kit Sou、Yuan Lu

展开 >

作者单位：

Key Laboratory of Industrial Biocatalysis,Ministry of Education,Tsinghua University,Beijing,100084,China

Department of Chemical Engineering,Tsinghua University,Beijing,100084,China

基金：

National Key R&D Program of ChinaNational Natural Science Foundation of ChinaInstitute Guo Qiang,Tsinghua UniversityDepartment of Chemical EngineeringiBHE Joint Cooperation Fund

项目编号：

2018 YFA0901700222782412021GQG1016

出版年：

2024

DOI：

10.1016/j.gee.2023.10.002

绿色能源与环境(英文)

CSTPCD

ISSN：

年,卷(期)：2024.9(9)