首页|钴氮共掺杂炭化木的制备及其降解罗丹明B性能研究

钴氮共掺杂炭化木的制备及其降解罗丹明B性能研究

扫码查看
钴基催化剂因其高催化活性而在水处理领域被广泛关注,然而循环稳定性低、分散性差等问题制约其应用.本研究通过聚多巴胺改性处理木材,浸渍钴盐溶液后再进行炭化,成功制备了钴氮共掺杂炭化木.结合X射线衍射、比表面积测定仪、拉曼光谱和扫描电子显微镜对其进行表征,并通过降解实验发现炭化木中的钴与掺氮炭层能够协同活化并产生活性物质(1O2,O·-2),在20 min内对罗丹明B的降解率可达99.60%.研究为炭化木基负载型催化剂的设计与制备提供思路.
Co/N Co-Doped Carbonized Wood for Rhodamine B Degradation
Cobalt-based catalysts have gained considerable attention in the field of water treatment due to the high catalytic activity.However,the application is hindered by challenges such as poor cycling stability and low dispersibility.This study successfully prepared cobalt-nitrogen co-doped carbonized wood through polydopamine modification treatment,followed by impregnation with cobalt salt solution and subsequent carbonization.The synthesized carbonized wood was characterized using X-ray diffraction,specific surface area analysis,Raman spectroscopy,and scanning electron microscopy.Degradation experiments revealed that the cobalt and nitrogen-doped carbon layers in the carbonized wood exhibited synergistic activation,achieving a 99.60%degradation of Rhodamine B within 20 minutes.The research provides insights on the design and preparation of carbonized wood-based supported catalysts.

carbonized woodnitrogen-doped carbon layerpolydopamine modificationdegradation performancecatalyst

曹志锋、刘苏玲、李连震、李雪琪、邢鹏宇、甘文涛

展开 >

东北林业大学材料科学与工程学院,黑龙江哈尔滨 150040

炭化木 掺氮炭层 聚多巴胺改性 降解性能 催化

中国科学技术协会青年人才托举工程国家自然科学基金

YESS2021003132001256

2023

木材科学与技术
中国林科院木材工业研究所

木材科学与技术

CSTPCD北大核心
影响因子:0.677
ISSN:2096-9694
年,卷(期):2023.37(5)
  • 11