首页|二维GO、MXene和MoS2限域离子液体复合膜用于碳捕集

二维GO、MXene和MoS2限域离子液体复合膜用于碳捕集

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工业化的急速发展导致大气中CO2的浓度急剧增加,给人类的生活带来了严重的威胁.因此,亟需发展碳捕集、利用与封存技术用于降低CO2的排放量.在多种方法中,膜分离技术逐渐成为全球碳捕集技术的主要发展方向.膜材料是膜的核心,随着新型制膜材料的不断涌现,一系列高性能气体分离膜层出不穷.离子液体(ILs)作为一种新型材料,因其在CO2分离过程中具有不易挥发、结构可调、对CO2有优异的亲和力等特点而备受欢迎.然而,由于ILs的高黏度和高成本限制了其在工业领域的应用.将ILs与二维纳米材料相结合,得到的新型复合膜兼具ILs和二维纳米材料的优势,可突破ILs的缺陷,成为未来膜材料的研究趋势之一.本综述以ILs为核心,重点介绍了将IL限域于二维氧化石墨烯(GO)、MXene和MoS2纳米材料的研究进展,讨论了 ILs的性质;总结了不同ILs与二维GO、MXene和MoS2材料所构建的气体分离膜在CO2捕获中的应用;讨论了 ILs在气体分离领域中的优势和挑战,并提出了未来的研究和发展机会.
Two-dimensional GO,MXene and MoS2 confined domain ionic liquid composite membranes for carbon capture
The rapid development of industrialization has led to a sharp increase in the concentration of CO2 in the atmosphere,posing a serious threat to human life.Therefore,there is an urgent need to develop carbon capture,utilization and sequestration(CCS)technologies to reduce CO2 emissions.Among various methods,membrane separation technology has gradually become the main development direction of global carbon capture technology.Membrane materials are the core of membranes,and a series of high-performance gas separation membranes have emerged with the continuous emergence of new membrane materials.Ionic liquids(ILs),as a new type of material,are popular in the CO2 separation process due to their non-volatile,adjustable structure and excellent affinity for CO2.However,the high viscosity and high cost of ILs limit the application of ILs in industry.However,the novel composite membrane obtained by combining ILs with 2D nanomaterials combines the advantages of both ILs and 2D nanomaterials,which can break through the defects of ILs and become one of the future research trends of membrane materials.For this reason,this review focuses on the research progress of limiting ILs to 2D GO,MXene and MoS2 nanomaterials with ILs as the core,and discusses the properties of ILs.In addition,the application of gas separation membranes constructed by different ILs with 2D GO,MXene and MoS2 materials in CO2 capture is presented.Finally,the advantages and challenges of ILs in gas separation are discussed,and future research and development opportunities are presented.

ionic liquidsmembrane separationCO2 capturetwo-dimensional nanomaterials

赵中源、侯铎、关鹏、黄国贤、周涛、李飞、骆文佳

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西北矿冶研究院,白银 730900

甘肃银光聚银化工有限公司,白银 730900

离子液体 膜分离 CO2捕获 二维纳米材料

甘肃省科技重大专项甘肃省重点研发计划项目

21ZD4GD03322YF7GD194

2024

膜科学与技术
中国蓝星(集团)股份有限公司

膜科学与技术

CSTPCD北大核心
影响因子:0.634
ISSN:1007-8924
年,卷(期):2024.44(4)
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