The origins of catalytic selectivity for the electrochemical conversion of carbon dioxide to methanol

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外文摘要：The electrocatalytic conversion of carbon dioxide(CO2)into useful fuels and chemical feedstocks is an emerging route to alleviate global warming and reduce reliance on fossil fuels.Methanol(CH3OH),as one of the most significant and widely used liquid fuels that can be generated by CO2 reduction,is essential in the chemical industry.In this minireview,we unravel the origins of the selective formation of CH3OH via CO2 reduction,including catalyst composition designs,local structure modulations,and electrolyte/catalyst interface regulations.Finally,the remaining challenges and perspectives for the CO2-to-CH3OH reduction are proposed.

外文关键词：

methanolcarbon dioxide(CO2)reduction reactionelectrochemistryelectrocatalystcatalyst-electrolyte interface

作者：

Tian Wang、Yating Wang、Yuhang Li、Chunzhong Li

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作者单位：

Key Laboratory for Ultrafine Materials of Ministry of Education,Shanghai Engineering Research Center of Hierarchical Nanomaterials,Frontiers Science Center for Materiobiology and Dynamic Chemistry,School of Materials Science and Engineering,East China University of Science &Technology,Shanghai 200237,China

School of Chemical Engineering,East China University of Science & Technology,Shanghai 200237,China

基金：

National Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaShanghai Municipal Science and Technology Major ProjectShanghai Scientific and Technological Innovation ProjectFundamental Research Funds for the Central Universities,Shanghai Rising-Star ProgramShanghai Sailing Program

项目编号：

22178104U22B20143218380032200806922dz120590023QA140220020YF1410200

出版年：

2024

DOI：

10.1007/s12274-023-5653-7

纳米研究(英文版)

CSTPCD

ISSN：

年,卷(期)：2024.17(1)

参考文献量92