首页|Advances of graphdiyne-supported metal catalysts in thermocatalytic reactions
Advances of graphdiyne-supported metal catalysts in thermocatalytic reactions
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Supported metal catalysts are widely used in the modern chemical industry.The electronic interaction between supports and active components is of great significance for heterogeneous catalysis.Graphdiyne(GDY),a new type of carbon allotrope with sp-hybridized carbon atoms,rr conjugate structure,and electron transmission capability,is a promising candidate as catalyst support.Recent years have witnessed the rapid progress of GDY-suppported metal catalysts for different catalysis reactions.Considering that most processes in the current chemical industry are thermocatalytic reactions,we herein give an overview about the advances and particular characteristics of GDY-supported catalysts in these reactions.The geometric structure and electronic properties of GDY are first introduced.Then,the synthesis methods for GDY-supported metal catalysts and their applications in thermocatalytic reactions are discussed,in which the effect of electronic interaction on catalytic performance is highlighted.Finally,the current challenges and future directions of GDY-supported metal catalysts for thermocatalysis are proposed.It is expected that this review will enrich our understanding of the advances of GDY as a superior support for metal catalysts in thermocatalytic reactions.
Jia Yu、Yida Yang、Yuliang Li、Changyan Cao、Weiguo Song
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Beijing National Laboratory for Molecular Sciences,CAS Research/Education Center for Excellence in Molecular Sciences,Laboratory of Molecular Nanostructures and Nanotechnology,Institute of Chemistry,Chinese Academy of Sciences,Beijing 100190,China
School of Chemical Sciences,University of Chinese Academy of Sciences,Beijing 100049,China
Beijing National Laboratory for Molecular Sciences,CAS Research/Education Center for Excellence in Molecular Sciences,Laboratory of organic solids,Institute of Chemistry,Chinese Academy of Sciences,Beijing 100190,China
National Key R&D Program of ChinaNational Key R&D Program of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaNational Natural Science Foundation of ChinaYouth Innovation Promotion Association of CAS
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