首页|石墨相氮化碳的异质结结构在光催化领域的研究进展

石墨相氮化碳的异质结结构在光催化领域的研究进展

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近年来,石墨相氮化碳(g-C3N4)因具有适宜的导带价带位置及低成本、低毒性、可见光驱动、稳定性好等特点在光驱动环境催化和新能源催化等领域受到广泛关注.然而,其光生电子-空穴对复合严重的问题,影响了石墨相氮化碳在各种光催化反应中的催化活性.由于石墨相氮化碳的异质结结构能够有效抑制光生电子-空穴对的复合并改善光生载流子的利用效率,因而其成为了光催化领域的研究热点.综述了过去5年中石墨相氮化碳的异质结结构在污染物光催化降解、光催化水分解产氢、二氧化碳光催化还原领域的研究进展,以期为石墨相氮化碳基材料在光催化领域的发展提供理论支持.
Research progress of graphite phase carbon nitride-based heterogeneous structure in the field of photocatalysis
In recent years,graphite phase carbon nitride(g-C3N4)has attracted much attention in the fields of light-driven environmental and new energy catalysis due to its suitable conduction and valence band position,low cost and toxicity,visible light response,as well as good stability.However,the serious problem of photogenerated electron-hole recombination has affected the catalytic activity of g-C3 N4 in various photocatalytic reactions.The heterostructure based on g-C3 N4 has become a research hotspot in the field of photocatalysis because it can suppress the photogenerated electron-hole pair recombination and improve the photogenerated carrier utilization efficiency.This article reviews the research progress of g-C3 N4 based heterojunction in the fields of pollutant photodegradation,photocatalytic water splitting for hydrogen production and photocatalytic carbon dioxide reduction in the past five years,which can provide theoretical support for the development of g-C3 N4 based materials in the field of photocatalysis.

g-C3N4heterojunctionpollutant photodegradationphotocatalytic water splittingcarbon dioxide photoreduction

王奕琛、勾思、赵震

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沈阳师范大学 化学化工学院,沈阳 110034

沈阳师范大学 能源与环境催化研究所,沈阳 110034

中国石油大学(北京)重质油国家重点实验室,北京 102249

g-C3N4 异质结 污染物光降解 光催化水分解 二氧化碳光还原

教育部"春晖计划"合作科研项目沈阳师范大学博士科研启动基金项目

HZKY20220426BS202016

2024

沈阳师范大学学报(自然科学版)
沈阳师范大学

沈阳师范大学学报(自然科学版)

CSTPCD
影响因子:0.591
ISSN:1673-5862
年,卷(期):2024.42(1)
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