首页|Recent advances in intermediate-temperature CO2 capture:Materials,technologies and applications

Recent advances in intermediate-temperature CO2 capture:Materials,technologies and applications

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Carbon capture,utilization and storage(CCUS)is widely recognized as a vital strategy for mitigating the impact of human induced climate change.Among various CO2 adsorbents,intermediate-temperature solid adsorbents have garnered significant attention due to their potential applications in hydrogen uti-lization,specifically in the water gas shift,steam reforming and gasification processes.These processes are crucial for achieving carbon neutrality.While laboratory-level studies have showcased the high adsorption capacity of these materials via various synthesis and modification methods,their practical application in complex industrial environments remains challenging,impeding the commercialization process.This review aims to critically summarize the recent research progress made in intermediate-temperature(200-400 ℃)solid CO2 adsorbents,particularly focusing on indicators such as cyclability,gas selectivity,and formability,which play vital roles in industrial application scenarios.Additionally,we provide an overview of laboratory-level advanced technologies specifically tailored for industrial applications.Furthermore,we highlight several industrial-ready advanced technologies that can pave the way for overcoming the challenges associated with large-scale implementation.The insights provided by this review aim to assist researchers in identifying the most relevant research directions for industrial applications.By promoting advances in the application of solid adsorbents,we strive to facilitate the ulti-mate goal of achieving carbon neutrality.

Intermediate-temperatureCO2 captureMgOLDHsIndustrialization

Chengbo Zhao、Leiming Wang、Liang Huang、Nicholas M.Musyoka、Tianshan Xue、Jabor Rabeah、Qiang Wang

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Engineering Research Center for Water Pollution Source Control & Eco-remediation,College of Environmental Science and Engineering,Beijing Forestry University,Beijing 100083,China

State Key Laboratory of Efficient Production of Forest Resources,Beijing Forestry University,Beijing 100083,China

China Machinery Huanyu Certification and Inspection Co.,Ltd.,Beijing 102609,China

Nottingham Ningbo China Beacons of Excellence Research and Innovation Institute,University of Nottingham Ningbo China,Ningbo 315100,Zhejiang,China

Institute of Atmospheric Environment,Chinese Research Academy of Environmental Sciences,Beijing 100012,China

Leibniz-Institut für Katalyse e.V.,Albert-Einstein-Str.29a,Rostock D-18059,Germany

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国家重点研发计划国家自然科学基金国家自然科学基金中央高校基本科研业务费专项

2022YFB410170252106072522250032019JQ03015

2024

10.1016/j.jechem.2023.11.024

能源化学
中国科学院大连化学物理研究所 中国科学院成都有机化学研究所

能源化学

CSTPCDEI
影响因子：0.654
ISSN：2095-4956
年,卷(期)：2024.90(3)
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