首页|Towards advanced zinc anodes by interfacial modification strategies for efficient aqueous zinc metal batteries

Towards advanced zinc anodes by interfacial modification strategies for efficient aqueous zinc metal batteries

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Developing sustainable and clean energy sources(e.g.,solar,wind,and tide energy)is essential to achieve the goal of carbon neutrality.Due to the discontinuous and inconsistent nature of common clean energy sources,high-performance energy storage technologies are a critical part of achieving this target.Aqueous zinc metal batteries(AZMBs)with inherent safety,low cost,and competitive performance are regarded as one of the promising candidates for grid-scale energy storage.However,zinc metal anodes(ZMAs)with irreversible problems of dendrite growth,hydrogen evolution reaction,self-corrosion,and other side reactions have seri-ously hindered the development and commercialization of AZMBs.An increasing number of researchers are focusing on the stability of ZMAs,so assessing the effectiveness of existing research strategies is critical to the development of AZMBs.This review aims to provide a comprehensive overview of the fundamentals and challenges of AZMBs.Research strategies for interfacial modification of ZMAs are systematically presented.The features of artificial interfacial coating and in-situ interfacial coating of ZMAs are compared and dis-cussed in detail,as well as the effect of modified interfacial ZMA on the full-battery performance.Finally,per-spectives are provided on the problems and challenges of ZMAs.This review is expected to offer a constructive reference for the further development and commercialization of AZMBs.

Aqueous zinc metal batteriesZinc metal anodeInterfacial modificationArtificial interfacial coatingIn-situ interfacial coating

Changchun Fan、Weijia Meng、Jiaye Ye

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Key Laboratory of Bio-Inspired Smart Interfacial Science and Technology,Ministry of Education,School of Chemistry,Beihang University,Beijing 100191,China

Shaanxi Key Laboratory of New Transportation Energy and Automotive Energy Saving,School of Energy and Electrical Engineering Chang'an University,Xi'an 710061,Shaanxi,China

School of Chemistry and Physics,Faculty of Science,Queensland University of Technology,Brisbane,QLD 4001,Australia

Centre for Materials Science,Queensland University of Technology,Brisbane,QLD 4001,Australia

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Australian Research Council,Centre for Materials Science,Queensland University of TechnologyFundamental Research Funds for the Central Universities,CHDX.Meng at Tianjin University of Science and Technology

2024

10.1016/j.jechem.2023.12.054

能源化学
中国科学院大连化学物理研究所 中国科学院成都有机化学研究所

能源化学

CSTPCDEI
影响因子：0.654
ISSN：2095-4956
年,卷(期)：2024.93(6)
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