首页|Engineering electrolyte additives for stable zinc-based aqueous batteries:Insights and prospects

Engineering electrolyte additives for stable zinc-based aqueous batteries:Insights and prospects

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Zn-based aqueous batteries(ZABs)are gaining widespread popularity due to their low cost and high safety profile.However,the application of ZABs faces significant challenges,such as dendrite growth and parasitic reactions of metallic Zn anodes.Therefore,achieving high-energy-density ZABs necessitates addressing the fundamental thermodynamics and kinetics of Zn anodes.Various strategies are available to mitigate these challenges,with electrolyte additive engineering emerging as one of the most efficient and promising approaches.Despite considerable research in this field,a comprehensive understanding of the intrinsic mechanisms behind the high performance of electrolyte additives remains limited.This review aims to provide a detailed introduction to functional electrolyte additives and thoroughly explore their underlying mechanisms.Additionally,it discusses potential directions and perspectives in additive engineering for ZABs,offering insights into future development and guidelines for achieving high-performance ZABs.

Aqueous batteriesZn anodesElectrolyte additive engineeringInterfacial chemistryElectrochemical mechanisms

Tao Liu、Xusheng Dong、Bin Tang、Ruizheng Zhao、Jie Xu、Hongpeng Li、Shasha Gao、Yongzheng Fang、Dongliang Chao、Zhen Zhou

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Interdisciplinary Research Center for Sustainable Energy Science and Engineering(IRC4SE2),Engineering Research Center of Advanced Functional Material Manufacturing of Ministry of Education,School of Chemical Engineering,Zhengzhou University,Zhengzhou 450001,Henan,China

Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education),Nankai University,Tianjin 300071,China

Laboratory of Advanced Materials,Shanghai Key Laboratory of Molecular Catalysis and Innovative Materials,State Key Laboratory of Molecular Engineering of Polymers and School of Chemistry and Materials,Fudan University,Shanghai 200433,China

College of Mechanical Engineering,Yangzhou University,Yangzhou 225127,Jiangsu,China

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2024

10.1016/j.jechem.2024.06.036

能源化学
中国科学院大连化学物理研究所 中国科学院成都有机化学研究所

能源化学

CSTPCDEI
影响因子：0.654
ISSN：2095-4956
年,卷(期)：2024.98(11)