同位素2024,Vol.37Issue(5) :455-462.DOI:10.7538/tws.2024.youxian.068

面向PGNAA技术的碘化钠探测器MCNP模拟计算

MCNP Simulation of NaI Detector for PGNAA Technology

王泽亮 贾文宝 杨晓艳 张镇华 张焱 程璨
同位素2024,Vol.37Issue(5) :455-462.DOI:10.7538/tws.2024.youxian.068

面向PGNAA技术的碘化钠探测器MCNP模拟计算

MCNP Simulation of NaI Detector for PGNAA Technology

王泽亮 1贾文宝 1杨晓艳 2张镇华 1张焱 3程璨4
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作者信息

  • 1. 南京航空航天大学,南京 211106
  • 2. 内蒙古自治区计量测试研究院,呼和浩特 010030
  • 3. 东华理工大学,南昌 330013
  • 4. 南京航空航天大学,南京 211106;南京工业大学,南京 210023
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摘要

碘化钠(NaI)探测器因其优秀的探测效率和相对较低的成本在瞬发γ射线中子活化分析技术(prompt gamma-ray neutron activation analysis,PGNAA)中具有广泛应用.为了获取PGNAA测量过程中探测器对γ射线的响应,针对NaI探测器建立了蒙特卡罗模型,基于该模型对中子以及γ射线输运过程进行模拟计算.对60Co、137Cs、152Eu、133Ba和241Am标准点源以及137Cs水体源进行了测量分析,并与MCNP模拟计算进行对比,结果显示两者吻合.之后结合D-D中子发生器对水溶液进行测量,并分析H元素辐射俘获反应产生的 2.223 MeV特征γ射线.研究结果表明,MCNP模拟计算的H元素特征峰计数与测量的结果偏差为 13%,证明了MCNP建立的NaI测量系统模型能够实现对γ和中子混合输运过程的模拟仿真,可为后续系统优化工作的开展奠定基础.

Abstract

Sodium iodide(NaI)detector has wide applications in Prompt Gamma-ray Neutron Activation Analysis(PGNAA)due to its excellent detection efficiency and relatively low cost.In order to obtain the response of the detector to gamma-rays during PGNAA measurement process,a Monte Carlo model was established for the NaI detector to simulate the transport processes of neutrons and gamma-rays.Measurements and analyses were conducted on standard point sources of 60Co,137Cs,152Eu,133Ba,and 241Am,as well as a waterborne source of 137Cs.These measurements were compared with MCNP simulation calculations,and the results demonstrated agreement between the two methodologies.Then,measurements were conducted on aqueous solutions using a D-D neutron generator,and the 2.223 MeV characteristic gamma-ray produced by the H element radiative capture reaction was analyzed.The research results show that the deviations between MCNP simulation calculations of characteristic peaks for the H element and experimental measurements were consistently within 13%,demonstrating that the NaI measurement system model established by MCNP can simulate the transport processes of gamma and neutrons,laying a foundation for the subsequent optimization of the system and other related work.

关键词

NaI探测器/MCNP模拟/瞬发γ射线能谱/中子输运

Key words

NaI detector/MCNP simulation/prompt gamma-ray spectrum/neutron transport

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基金项目

国家自然科学基金项目(12105143)

国家自然科学基金项目(42374226)

国家重点研发计划(2023YFF0717003)

江西省自然科学基金项目(2023BAB201043)

江西省自然科学基金项目(20232BCJ23006)

江苏省市场监督管理局科技计划项目(KJ2024009)

江苏省市场监督管理局科技计划项目(KJ2024044)

江苏省市场监督管理局科技计划项目(KJ2023015)

放射医疗协同创新中心项目(YF202301)

出版年

2024
同位素
中国核学会同位素分会

同位素

CSTPCD
影响因子:0.405
ISSN:1000-7512
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