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飞秒激光诱发Ni及其异质结薄膜的太赫兹辐射测量

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采用磁控溅射法在SiO2基底上生长厚度均为10 nm的Ni膜、Ni/Pt和CoFeB/Ni双层异质结薄膜,并测量3种薄膜在飞秒脉冲激光激发下的太赫兹发射谱.通过频谱分析发现,这3种Ni薄膜的太赫兹辐射主要来源于超快自旋-电荷的转换,且不同结构的转换机制不同.对于单层Ni薄膜,太赫兹辐射主要来源于Ni的超快退磁和异常霍尔效应;对于Ni/Pt双层膜,此时Ni起自旋注入作用,由Pt完成自旋-电荷转换而产生太赫兹信号;对于CoFeB/Ni双层膜,自旋电流由CoFeB产生,而Ni起自旋-电荷转换作用.通过飞秒激光-太赫兹技术,可以研究铁磁Ni材料的磁学特性.
Measuring terahertz radiation from Ni and its heterojunction thin films by femtosecond laser
Ni film,Ni/Pt bilayer and CoFeB/Ni bilayer heterojunction with a thickness of 10 nm were grown on SiO2 substrates by magnetron sputtering,and their terahertz emission spectra excited by femtosecond laser technology were measured.Through spectral analysis,it was found that the ter-ahertz radiation of these three kinds of Ni films mainly came from the ultrafast spin-to-charge conver-sion,and the conversion mechanism was different for different structures.For single-layer Ni films,terahertz radiation was mainly due to the ultrafast demagnetization of Ni and the anomalous Hall effect.For the Ni/Pt bilayer,Ni played the role of spin injection,and the Pt completed the spin-to-charge conversion to generate a terahertz signal.For CoFeB/Ni bilayer,the spin current was genera-ted by CoFeB,and Ni played the role of spin-to-charge conversion.The magnetic properties of ferro-magnetic Ni materials could be studied by the femtosecond laser-terahertz technology.

Ni nanofilmsheterojunction nanofilmsfemtosecond laser technologyterahertz e-mission spectraspin-to-charge conversion

卫翼、方铄、李恒一

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中国科学技术大学化学与材料科学学院,安徽 合肥 230026

中国科学技术大学物理学院,安徽 合肥 230026

Ni薄膜 异质结薄膜 飞秒激光技术 太赫兹发射谱 自旋-电荷转换

2024

物理实验
东北师范大学

物理实验

影响因子:0.573
ISSN:1005-4642
年,卷(期):2024.44(12)