首页|基于表面等离激元的新型碲化铯光阴极研究

基于表面等离激元的新型碲化铯光阴极研究

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目前已有研究将表面等离极化激元(SPPs)引入铜阴极和锑钾铯光阴极中,大幅提高其量子效率。碲化铯(Cs2Te)光阴极是一种极佳的在紫外频段可应用于中高平均流强的光阴极材料,而常用贵金属介电函数在紫外频段过低无法满足SPPs激发要求。本研究通过微纳光栅结构将SPPs引入Cs2Te光阴极,形成局域增强场以提高光子吸收率,并调节光电子初始激发分布。为探索SPPs对Cs2Te光阴极性能的影响,使用蒙特卡罗方法模拟引入SPPs前后光阴极的光电发射过程。结果表明,引入SPPs会导致光电子数量增加,从而显著提高Cs2Te光阴极的量子效率约60%,且增加的光电子大多数分布于深层界面附近,在逃逸过程中各类碰撞概率增加,使发射度基本保持不变。
Studies on Novel Cs2Te Photocathode Based on Surface Plasmon Polaritons
Cathodes serve as sources of electron beams,and their performance plays a great part of beam quality in electron accelerators.The introduction of surface plasmon polaritons(SPPs)into different photocathodes has been investigated to increase their quantum efficiency.Currently,the SPPs excitation is predominantly achieved in the infrared and visible bands due to limitations in the permittivity of common noble metals.Exciting SPPs in the ultraviolet band typically involve attaching aluminium nano-particles to the material surface,which can impact the optical properties of the material.Therefore,it is important to develop a method for exciting SPPs in the ultraviolet band without affecting optical properties of the material.The cesium telluride(Cs2Te)photocathode represents a lifetime of several months,a quantum efficiency of up to 10%,a response time of less than 1 ps,a thermal emittance of less than 1 mm·mrad/mm,and moderate operating vacuum requirement of 10-7 Pa.These characteristics make Cs2Te an exceptional photocathode material for generating high-current electron beams.However,a drawback of Cs2Te photocathodes is that they need to be excited by high-power ultraviolet lasers,which are more challenging to obtain compared to green lasers.Consequently,there is a continued demand for increasing the quantum efficiency of Cs2Te to reduce the laser power requirements.In this paper,accuracy of the Monte Carlo model to simulate the Cs2Te photoemission was verified.SPPs were introduced into Cs2Te photocathode by means of micro-nano grating structure,which increases substantially the absorption of incident photons and hence form a local field enhancement to regulate initial photoelectrons distribution.The Monte Carlo model was modified according to the theory of SPPs to simulate the photoelectric emission process of the Cs2Te photocathode after the introduction of SPPs.The simulation results show that the quantum efficiency of Cs2Te photocathode increases by 60%while the thermal emittance is basically unchanged,with the introduction of SPPs.This is due to the photoelectrons population,resulting from the additional laser absorption induced by the SPPs,decreases exponentially from the Cs2Te/Al interface to the vacuum/Cs2Te interface.The majority of these increased photoelectrons are distributed near the deeper interface,resulting in higher scattering probabilities during their transport from inside the photocathode to the surface,leading to a reduction of thermal emittance of the emitted electrons.Combined with conventional methods for controlling the thermal emittance of photocathodes,such as reducing the energy of incident laser photons and operating at low temperatures,it is anticipated that a photocathode with higher performance,characterized by low thermal emittance and high quantum efficiency,can be achieved.This advancement holds significant implications for the future development of high-brightness electron sources.

Cs2Te photocathodeultraviolet bandsurface plasmon polaritonsquantum efficiencythermal emittance

刘子硕、戴责已、关家宝、刘兰忻、钟建华、姜增公、王纪科、聂元存

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武汉大学高等研究院,湖北武汉 430072

中国科学院上海高等研究院,上海 201210

碲化铯光阴极 紫外频段 表面等离极化激元 量子效率 热发射度

国家自然科学基金面上项目

12275196

2024

原子能科学技术
中国原子能科学研究院

原子能科学技术

CSTPCD北大核心
影响因子:0.372
ISSN:1000-6931
年,卷(期):2024.58(10)