首页|Photocatalytic Methane Conversion:Insight into the Mechanism of C(sp3)-H Bond Activation
Photocatalytic Methane Conversion:Insight into the Mechanism of C(sp3)-H Bond Activation
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Mild and direct conversion of methane into high value-added products is a desired goal for chemistry,energy,and environment.The active species gener-ated in the photocatalytic reaction system under mild conditions activate the inert C-H bond in meth-ane and promote methane conversion.This review focuses on the developed mechanisms for C(sp3)-H bond activation in photocatalytic methane conver-sion,including radical and active site mechanisms.Particular emphasis is placed on the detailed sum-mary of mechanism,characterization method,and corresponding application in photocatalytic meth-ane conversion.We also discuss the challenges and prospects for future direction on C(sp3)-H bond activation mechanism in photocatalytic methane conversion.This review aims to promote the devel-opment of photocatalytic methane conversion and provides guidance for the design of high-efficiency photocatalysts.
photocatalysismethaneC-H bondsrad-icalactive site
Yuheng Jiang、Yingying Fan、Siyang Li、Zhiyong Tang
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Chinese Academy of Science(CAS)Key Laboratory of Nanosystem and Hierarchy Fabrication,CAS Center for Excellence in Nanoscience,National Center for Nanoscience and Technology,Beijing 100190
Center for Nanoscale Science and Technology,Academy for Advanced Interdisciplinary Studies,Peking University,Beijing 100871
University of Chinese Academy of Sciences,Beijing 100049
Center for Advanced Analytical Science,School of Chemistry and Chemical Engineering,School of Civil Engineering,Analytical and Testing Center,Guangzhou University,Guangzhou 510006
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中国科学院战略规划重点项目中国科学院战略规划重点项目国家重点基础研究发展计划(973计划)国家重点基础研究发展计划(973计划)国家自然科学基金国家自然科学基金国家自然科学基金国家自然科学基金Guangdong Basic and Applied Basic Research FoundationGuangdong Basic and Applied Basic Research FoundationOncampus Scientifc Research Project of Guangzhou UniversityOncampus Scientifc Research Project of Guangzhou University
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