首页|Probing On-Surface Chemistry at the Nanoscale Using Tip-Enhanced Raman Spectroscopy
Probing On-Surface Chemistry at the Nanoscale Using Tip-Enhanced Raman Spectroscopy
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Chemistry on solid surfaces is central to many re-search areas of practical interest,such as synthesis,catalysis,electrochemistry,photochemistry,and materials science.A comprehensive understanding of the nanoscale on-surface chemistry involved in these areas is important for establishing composi-tion-structure-performance relationships.With the rapid development of tip-enhanced Raman spectros-copy(TERS),it has become possible to investigate physical and chemical processes on suitable surfaces at the nanoscale level and in real space.In this review,after a brief introduction of the background of on-surface chemistry and TERS,we systematically dis-cuss the progress in the application of TERS in this field.Our focus is the applications of TERS to nano-scale coordination processes,decomposition reac-tions,polymerization processes,electrochemical reactions,catalytic chemistry,and functionalization chemistry on solid surfaces.We conclude by discuss-ing the future challenges and development of TERS techniques and related applications in on-surface chemistry.
on-surface chemistrytip-enhanced Raman spectroscopyscanning probe microscopychemical imagingnanoscale chemical analysisspa-tial resolution
Zhen-Feng Cai、Naresh Kumar、Renato Zenobi
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Department of Chemistry and Applied Biosciences,ETH Zurich,Zurich CH-8093
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