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Advances in Electrochemical Oxidation of Olefins to Epoxides
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Epoxides are important chemicals and used in multi-ple fields.The conventional thermal-catalytic produc-tion of epoxides consumes a large amount of energy and generates abundant carbon emissions.Therefore,sustainable manufacturing technologies are highly desired.Taking advantage of renewable electricity to drive electrochemical epoxidation reactions provides a novel approach to generating value-added products in the chemicals sector.This review describes the current progress of selective electrochemical oxida-tion of olefins to epoxides,which is categorized according to the different reaction mechanisms.The halide-mediated method is first discussed,followed by an overview of electrochemical epoxidations with H2O and O2-derived H2O2.Moreover,the existing problems in this fast-growing field and future devel-oping directions are pointed out.This review hopes to provide inspiration for the design of electrocatalysts,electrode materials,and electrolyzers for the electro-chemical production of epoxides in a sustainable manner.
Key Laboratory for Green Chemical Technology of Ministry of Education,School of Chemical Engineering and Technology,Tianjin University,Tianjin 300072
Collaborative Innovation Center of Chemical Science and Engineering(Tianjin),Tianjin 300072
National Industry-Education Platform of Energy Storage,Tianjin University,Tianjin 300350
Haihe Laboratory of Sustainable Chemical Transformations,Tianjin 300192
Joint School of National University of Singapore and Tianjin University,International Campus of Tianjin Unive
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国家重点研发计划国家自然科学基金国家自然科学基金国家自然科学基金Haihe Laboratory of Sustainable Chemical TransformationsProgram of Introducing Talents of Discipline to UniversitiesXplorer Prize for financial support
NETL
NSTL
万方数据
维普
