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高能超宽带光参量啁啾脉冲放大过程中的空间相位演变特性研究

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基于高掺氘DKDP晶体的光参量啁啾脉冲放大(OPCPA)技术是实现百拍瓦(100 PW)超强超短激光脉冲放大的主要技术路线之一。基于SEL-100 PW激光装置OPCPA高能主放大系统的设计,研究了高能量泵浦光的空间近场分布和相位分布对高能量、超宽带OPCPA过程中信号光空间相位演变特性的影响。仿真计算结果表明:在非共线O PCPA过程中,信号光空间相位分布的变化主要由泵浦光空间强度分布和相位分布引起;在严格的相位匹配条件下,泵浦光光强呈6阶超高斯分布,当低阶相位畸变为1λ时,放大信号光的空间相位畸变为10-2~10-4 rad,该值可以忽略,而且信号光相位空间分布与泵浦光相位空间分布梯度线性相关;在相位失配条件下,泵浦光光强将严重影响信号光的空间相位分布。本研究结果为基于高能、超宽带OPCPA技术路线的100 PW激光放大和波前优化提供了理论支持。
Spatial Phase Evolution Characteristics in the Process of High-Energy Ultra-Wideband OPCPA
Objective Ultra-short ultra-intense lasers can provide unprecedented extreme physical conditions and new experimental methods,leading to significant applications in laser acceleration,plasma physics,strong field physics,and high-energy density physics.OPCPA technology is an important method for realizing ultrashort laser amplification.Currently,the highest output peak power based on OPCPA technology is up to 4.9 PW.To further increase the peak power,larger-size crystals are required,and the gain spectrum width can be compressed to tens of femtoseconds.The extreme light physical line station(SEL),an integral part of the hard X-ray free electron laser(SHINE)project,a significant national science and technology infrastructure in China,is undertaking the construction of an ultra-short and ultra-intense laser(SEL-100 PW),aiming for a remarkable peak power of 100 PW.The interaction between the ultra-high focused intensity produced by a 100 PW laser and hard X-ray free electron laser is used to explore the strong field quantum electrodynamics(QED)and other frontier science and technology fields.For ultra-intense and ultra-short laser-matter interaction experiments,the focused peak power density(focused intensity)of the laser is one of the most important technical indexes,which requires ultra-high peak laser power and a focused focal spot close to the diffraction limit level.The ability of a laser to focus near the diffraction limit is primarily limited by its spatial phase(wavefront)distortion.In addition to the static wavefront aberration introduced by optical component processing and mounting errors,dynamic wavefront aberration during the laser amplification process is also an important influencing factor.Additionally,the near-field spatial distribution of a laser beam determines the safety of high-energy lasers during transmission.To study the dynamic phase evolution of the 100 PW laser OPCPA high-energy main amplifier,this study focuses on the three-wave beam quality evolution in the process of OPCPA amplification.Furthermore,the influence of the intensity distribution and wavefront distribution of different pump light on the wavefront distortion of the amplified signal is studied.Methods Solving the three-wave coupling equation in the spatial domain is important for studying the spatial phase evolution characteristics in high-energy,ultra-wideband OPCPA processes.The split-step Fourier method is important for numerically solving the three-wave coupling equations.The basic idea was to divide the nonlinear crystal into multiple parts,in which the free propagation of light is considered first,and then the nonlinear effects were considered.Once a reasonable mathematical model was developed,the characteristics of the signal light under the experimental conditions of a 100 PW laser device were first calculated.Subsequently,the phase mismatch and intensity distribution of the pump light were considered.Furthermore,the effect of the spatial phase distribution and saturation effect of the pump light on the energy and spatial phase of the amplified signal was considered.Results and Discussions The energy of the amplified signal light can be obtained by simulating the experimental conditions of the 100 PW laser,and the spectrum and intensity distribution can satisfy the requirements of subsequent compression(energy>300 J,spectral range is 925 nm+100 nm)(Figs.2,3).First,the phase mismatch is analyzed,and it can be concluded that the phase mismatch has a significant influence on the conversion efficiency and PV value of the amplified signal light phase;therefore,phase matching is an important condition for determining the output performance of OPCPA.Subsequently,the influence of the spatial phase distribution of the pump light on the amplified signal light is analyzed,which is proportional to the spatial derivative of the defocus of the pump light and occurs only in one dimension of the nonlinear angle(Fig.6).The influence of the intensity distribution of the pump light on the amplified signal light is analyzed.The spatial distribution of the pump light is imprinted on the phase of the amplified signal light,which is evident in the single-directional linear modulation and central-region protrusions(Figs.9,10,11,12).Finally,the effect of the saturation effect on the amplified signal light is considered,and with a further increase in the pump energy,the signal light reaches saturation and the conversion efficiency decreases.The PV value of the amplified signal light phase also increases with the increase in energy,although the growth gradually decelerates(Fig.13).Conclusions It can be concluded that under the input condition of the amplifier stage,the output of ultrashort and ultra strong pulses on the order of 100 PW can be realized.The pump light phase experiences only a small overall change gradient due to the large spatial size of the pump light.Therefore,the phase distortion of the pump light has slight effect on the phase of the amplified signal,and the effect of the phase distortion of the pump light at the wavelength level of 10-4 can be neglected in the design process.However,in a phase mismatch,the intensity distortion of the pump light has a significant impact on the intensity and phase of the signal light.Hence,the intensity distribution and phase matching of the pump light are necessary to realize a high-quality ultrashort pulse output in the design process.In subsequent studies,we will also conduct validation experiments to verify the simulation results.

laser opticsoptical parametric chirped pulse amplification100 PWnumerical simulationwavefront distortion

薛普凯、王傲天、李进峰、於亮红、梁晓燕

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中国科学院上海光学精密机械研究所强场激光物理国家重点实验室,上海 201800

中国科学院大学材料科学与光电技术学院,北京 100049

激光光学 光学参量啁啾脉冲放大 百拍瓦 数值模拟 波前畸变

国家重大科技基础设施研究计划上海市领军人才资助项目国家自然科学基金中国科学院青年创新促进会资助项目上海市科委科技创新行动计划

2017YFE012370020SR01450111804349201924719142202500

2024

中国激光
中国光学学会 中科院上海光机所

中国激光

CSTPCD北大核心
影响因子:2.204
ISSN:0258-7025
年,卷(期):2024.51(11)